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Review | Open Access

Recent Advances on Challenges and Strategies of Manganese Dioxide Cathodes for Aqueous Zinc-Ion Batteries

Yuhui Xu^{¹^,²}, Gaini Zhang^{¹^,²}(), Jingqian Liu^{¹^,²}, Jianhua Zhang^{¹^,²}, Xiaoxue Wang^{¹^,²}, Xiaohua Pu^{¹^,²}, Jingjing Wang^{¹^,²}, Cheng Yan^{¹^,²}, Yanyan Cao^{¹^,²}, Huijuan Yang^{¹^,²}, Wenbin Li^{¹^,²}, Xifei Li^{¹^,²^,³}

()

1

Key Laboratory of Advanced Batteries Materials for Electric Vehicles of China Petroleum and Chemical Industry Federation, Institute of Advanced Electrochemical Energy & School of Materials Science and Engineering, Xi’an University of Technology, Xi’an 710048, China

2

Engineering Research Center of Conducting Materials and Composite Technology, Ministry of Education, Xi’an 710048, China

3

Center for International Cooperation on Designer Low-carbon & Environmental Materials (CDLCEM), Zhengzhou University, Zhengzhou 450001, China

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Abstract

Aqueous zinc-ion batteries (AZIBs) are regarded as promising electrochemical energy storage devices owing to its low cost, intrinsic safety, abundant zinc reserves, and ideal specific capacity. Compared with other cathode materials, manganese dioxide with high voltage, environmental protection, and high theoretical specific capacity receives considerable attention. However, the problems of structural instability, manganese dissolution, and poor electrical conductivity make the exploration of high-performance manganese dioxide still a great challenge and impede its practical applications. Besides, zinc storage mechanisms involved are complex and somewhat controversial. To address these issues, tremendous efforts, such as surface engineering, heteroatoms doping, defect engineering, electrolyte modification, and some advanced characterization technologies, have been devoted to improving its electrochemical performance and illustrating zinc storage mechanism. In this review, we particularly focus on the classification of manganese dioxide based on crystal structures, zinc ions storage mechanisms, the existing challenges, and corresponding optimization strategies as well as structure–performance relationship. In the final section, the application perspectives of manganese oxide cathode materials in AZIBs are prospected.

Keywords

aqueous zinc-ion batteries challenges manganese dioxide optimized strategies zinc storage mechanisms

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Energy & Environmental Materials

Volume 6 Issue 6,
November 2023

DOI: 10.1002/eem2.12575

Cite this article:

Xu Y, Zhang G, Liu J, et al. Recent Advances on Challenges and Strategies of Manganese Dioxide Cathodes for Aqueous Zinc-Ion Batteries. Energy & Environmental Materials, 2023, 6(6). https://doi.org/10.1002/eem2.12575

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