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We report the formation of high-quality Cs0.4MA0.6PbBr3 thin films with nearly full surface coverage and good emission properties upon the introduction of Cs+ into perovskite crystals. The Cs0.4MA0.6PbBr3 thin films were applied as emissive layers in light-emitting diodes. A maximum external quantum efficiency of ~2.0% was achieved for these green-emitting devices.
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