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Research Article

High yield production of ultrathin fibroid semiconducting nanowire of Ta2Pd3Se8

Xue Liu1,2, Sheng Liu2, Liubov Yu. Antipina3,5,6, Yibo Zhu7, Jinliang Ning1, Jinyu Liu1, Chunlei Yue1, Abin Joshy1, Yu Zhu4, Jianwei Sun1, Ana M. Sanchez8, Pavel B. Sorokin3,5, Zhiqiang Mao1, Qihua Xiong2, Jiang Wei1( )
Department of Physics and Engineering Physics, Tulane University, New Orleans, Louisiana 70118, USA
Division of Physics and Applied Physics, Nanyang Technological University, Singapore 637371, Singapore
National University of Science and Technology "MISiS", Moscow 119049, Russia
Department of Polymer Science, The University of Akron, Akron , Ohio44325, USA
Technological Institute for Superhard and Novel Carbon Materials, Moscow 108840, Russia
Moscow Institute of Physics and Technology, Dolgoprudny 141700, Russia
Department of Mechanical Engineering, Columbia University, New York, New York 10027, USA
Department of Physics, University of Warwick, Coventry, CV4 7AL, UK
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An erratum to this article is available online at:
https://doi.org/10.1007/s12274-020-2914-6

Graphical Abstract

Abstract

Immediately after the demonstration of the high-quality electronic properties in various two dimensional (2D) van der Waals (vdW) crystals fabricated with mechanical exfoliation, many methods have been reported to explore and control large scale fabrications. Comparing with recent advancements in fabricating 2D atomic layered crystals, large scale production of one dimensional (1D) nanowires with thickness approaching molecular or atomic level still remains stagnant. Here, we demonstrate the high yield production of a 1D vdW material, semiconducting Ta2Pd3Se8 nanowires, by means of liquid-phase exfoliation. The thinnest nanowire we have readily achieved is around 1 nm, corresponding to a bundle of one or two molecular ribbons. Transmission electron microscopy (TEM) and transport measurements reveal the as-fabricated Ta2Pd3Se8 nanowires exhibit unexpected high crystallinity and chemical stability. Our low-frequency Raman spectroscopy reveals clear evidence of the existing of weak inter-ribbon bindings. The fabricated nanowire transistors exhibit high switching performance and promising applications for photodetectors.

Keywords

van der Waals nanowire1D semiconductorliquid exfoliationmicro Raman spectroscopyelectronic and optoelectronic device

Electronic Supplementary Material

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12274_2020_2784_MOESM1_ESM.pdf (3.5 MB)

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Nano Research
Volume 13 Issue 6,
June 2020
Pages 1627-1635
DOI: 10.1007/s12274-020-2784-y
Cite this article:
Liu X, Liu S, Yu. Antipina L, et al. High yield production of ultrathin fibroid semiconducting nanowire of Ta2Pd3Se8. Nano Research, 2020, 13(6): 1627-1635. https://doi.org/10.1007/s12274-020-2784-y
Topics:
CrystallinityCrystalsElectronic propertiesFabricationHigh resolution transmission electron microscopyNanowiresPalladium compoundsSelenium compoundsTantalum compoundsVan der Waals forces

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Received: 23 December 2019
Revised: 03 March 2020
Accepted: 31 March 2020
Published: 12 May 2020
© Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2020
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