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Research Article

Transparent, stretchable, temperature-stable and self-healing ionogel-based triboelectric nanogenerator for biomechanical energy collection

Weiqiang Liao1,§, Xiukun Liu1,§, Yuqi Li1( ), Xu Xu1, Jinxing Jiang2, Shaorong Lu1, Dequan Bao2, Zhen Wen2( ), Xuhui Sun2( )
Key Laboratory of New Processing Technology for Nonferrous Metals and Materials, Ministry of Education, College of Materials Science and Engineering, Guilin University of Technology, Guilin 541004, China
Institute of Functional Nano and Soft Materials (FUNSOM), Jiangsu Key Laboratory for Carbon-Based Functional Materials and Devices, Soochow University, Suzhou 215123, China

§Weiqiang Liao and Xiukun Liu contributed equally to this work.

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Graphical Abstract

Abstract

A flexible and stable power supply is essential to the rapid development of wearable electronic devices. In this work, a transparent, flexible, temperature-stable and ionogel electrode-based self-healing triboelectric nanogenerator (IS-TENG) was developed. The ionogel with excellent stretchability (1,012%), high ionic conductivity (0.3 S·m−1) and high-temperature stability (temperature range of −77 to 250 °C) was used as the electrode of the IS-TENG. The IS-TENG exhibited excellent transparency (92.1%) and stability. The output performance did not decrease when placed in a 60 °C oven for 48 h. In addition, the IS-TENG behaved like a stable output in the range of −20 to 60 °C. More importantly, the IS-TENG could also achieve self-healing of electrical performance at temperatures between −20 and 60 °C and its output can be restored to its original state after healing. When the single-electrode IS-TENG with an area of 3 cm × 3 cm was conducted under the working frequency of 1.5 Hz, the output values for open-circuit voltage, short-circuit current, short-circuit transferred charge, and maximum peak power density were 189 V, 6.2 μA, 57 nC, and 2.17 W·m−2, respectively. The IS-TENG enables to harvest biomechanical energy, and drive electronic devices. Furthermore, the application of IS-TENGs as self-driven sensors for detecting human behavior was also demonstrated, showing good application prospects in the field of wearable power technology and self-driven sensing.

Keywords

triboelectric nanogeneratorstretchableself-healingionogeltemperature-stable

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Nano Research
Volume 15 Issue 3,
March 2022
Pages 2060-2068
DOI: 10.1007/s12274-021-3797-x
Cite this article:
Liao W, Liu X, Li Y, et al. Transparent, stretchable, temperature-stable and self-healing ionogel-based triboelectric nanogenerator for biomechanical energy collection. Nano Research, 2022, 15(3): 2060-2068. https://doi.org/10.1007/s12274-021-3797-x
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Received: 02 May 2021
Revised: 07 August 2021
Accepted: 09 August 2021
Published: 07 September 2021
© Tsinghua University Press and Springer-Verlag GmbH Germany, part of Springer Nature 2021
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