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Research Article

Pomegranate micro/nano hierarchical plasma structure for superior microwave absorption

Chunyan Ding1,4, Tao Wu1( ), Xinsen Hu1, Chengshuai Shao1, Zhipeng Xu1, Hui Fu1, Songsong Wu1,3( ), Guangwu Wen1,3,4, Xiaoxiao Huang2( )
School of Materials Science and Engineering, Shandong University of Technology, Zibo 255000, China
School of Materials Science and Engineering, Harbin Institute of Technology, Harbin 150001, China
Shandong Industrial Ceramics Research & Design Institute Co., Ltd., Zibo 255000, China
Shandong Institute of Advanced Ceramic Co., Ltd., Zibo 255000, China
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Graphical Abstract

VSe2−x presents stronger adsorption towards lithium polysulfides due to selenium vacancies and shows the bidirectional catalysis towards the sulfur redox reactions.

Abstract

Inspired by the pomegranate natural artful structure, pomegranate micro/nano hierarchical plasma configuration of Fe/Fe3C@graphitized carbon (FFC/pCL) was constructed based on the green sol-gel method and in-situ chemical vapor deposition (CVD) synthesis protocol. Pomegranate-like FFC/pCL successfully overcame the agglomeration phenomenon of magnetic nanoparticles with each seed of the pomegranate consisting of Fe/Fe3C as cores and graphitized carbon layers as shells. The high-density arrangement of magnetic nanoparticles and the design of pomegranate-like heterostructures lead to enhanced plasmon resonance. Thus, the pomegranate-like FFC/pCL achieved a great electromagnetic wave (EMW) absorbing performance of 6.12 GHz wide band absorption at a low mass adding of only 16.7 wt.%. Such excellent EMW performance can be attributed to its unique pomegranate hierarchical plasma configuration with separated nanoscale iron cores, surface porous texture, and good carbon conductive network. This investigation provides a new paradigm for the development of magnetic/carbon based EMW absorbing materials by taking advantage of pomegranate hierarchical plasma configuration.

Keywords

electromagnetic wave absorptionlow filler loadingcarbon shellnetwork structuremagnetic Fe/Fe3C

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Nano Research
Volume 15 Issue 10,
October 2022
Pages 8688-8696
DOI: 10.1007/s12274-022-4522-0
Cite this article:
Ding C, Wu T, Hu X, et al. Pomegranate micro/nano hierarchical plasma structure for superior microwave absorption. Nano Research, 2022, 15(10): 8688-8696. https://doi.org/10.1007/s12274-022-4522-0
Topics:
Carbon composites

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Received: 26 February 2022
Revised: 09 May 2022
Accepted: 10 May 2022
Published: 02 August 2022
© Tsinghua University Press 2022
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