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Review Article

Realizing high-performance all-solid-state batteries with sulfide solid electrolyte and silicon anode: A review

Xinyang Wang1,2, Kuang He3, Siyuan Li1,2, Jiahui Zhang1,2, Yingying Lu1,2( )
State Key Laboratory of Chemical Engineering, Institute of Pharmaceutical Engineering, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou 310027, China
ZJU-Hangzhou Global Scientific and Technological Innovation Center, Hangzhou 311215, China
Zhejiang Yongtai Technology Co., Ltd., Taizhou 317000, China
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Graphical Abstract

To realize high-performance all-solid-state batteries with sulfide solid electrolytes (SEs) and silicon anodes, we introduce the critical bulk properties of sulfide SEs and the most recent improving strategies covering the ionic conductivity, electrochemical window, air stability, mechanical stability, thermostability and solvent stability. The main factors affecting the compatibility of silicon and sulfide SE, including the carbon’s effect, particle size of silicon, pressure and sulfide’ modules, silicon composite matrix, and depth of silicon’s lithiation are also elaborated in detail.

Abstract

Sulfide solid electrolyte (SE) is one of the most promising technologies for all-solid-state batteries (ASSBs) because of its high ionic conductivity and ductile mechanical properties. In order to further improve the energy density of sulfide-based ASSBs and promote practical applications, silicon anodes with ultrahigh theoretical capacity (4,200 mAh·g−1) and rich resource abundance have broad commercial prospects. However, significant challenges including bulk instability of sulfide SEs and poor utilization of silicon materials have severely impeded the ASSBs from becoming viable. In this review, we first introduce the critical bulk properties of sulfide SEs and the most recent improving strategies covering the ionic conductivity, air stability, electrochemical window, mechanical stability, thermostability and solvent stability. Next, we introduce the main factors affecting the compatibility of silicon and sulfide SE, including the carbon’s effect, particle size of silicon, external pressure, silicon composite matrix and the depth of silicon’s lithiation. Finally, we discuss possible research directions in the future. We hope that this review can provide a comprehensive picture of the role of nanoscale approaches in recent advances in ASSBs with sulfide and silicon, as well as a source of inspiration for future research.

Keywords

all-solid-state batterysulfide solid electrolytesilicon anodenanoscale optimization

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Nano Research
Volume 16 Issue 3,
March 2023
Pages 3741-3765
DOI: 10.1007/s12274-022-4526-9
Cite this article:
Wang X, He K, Li S, et al. Realizing high-performance all-solid-state batteries with sulfide solid electrolyte and silicon anode: A review. Nano Research, 2023, 16(3): 3741-3765. https://doi.org/10.1007/s12274-022-4526-9
Topics:
Electric energy storageLithium batteries
Part of a topical collection:
Women’s Special Issue: Nanomaterials: Preparation, Applications, and ChallengesWomen’s special issuse in nanomaterials

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Received: 14 March 2022
Revised: 06 May 2022
Accepted: 11 May 2022
Published: 26 July 2022
© Tsinghua University Press 2022
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