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Research Article

Three-dimensional MXene-encapsulated porous Ni-NDC nanosheets as anodes for enhanced lithium-ion batteries

Yuxin Shi1,§, Guoyin Zhu2,§, Xiaotian Guo1, Qingling Jing1, Huan Pang1( ), Yizhou Zhang2( )
School of Chemistry and Chemical Engineering, Yangzhou University, Yangzhou 225002, China
Institute of Advanced Materials and Flexible Electronics (IAMFE), School of Chemistry and Materials Science, Nanjing University of Information Science and Technology (NUIST), Nanjing 210044, China

§ Yuxin Shi and Guoyin Zhu contributed equally to this work.

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Graphical Abstract

The MXene-encapsulated porous Ni-naphthalene dicarboxylic acid (Ni-NDC) nanosheets exhibit reversible discharge capacity and good long-term cycling performance, owing to the synergistic effects between Ni-NDC and MXene. The strategy of fabricating metal–organic framework (MOF)-based composites offers an idea to prepare low-cost as well as efficient anode materials in lithium-ion batteries (LIBs).

Abstract

Although metal–organic frameworks have been heavily tested as the anode materials for lithium-ion batteries (LIBs), the poorer conductivity, easy collapse of frameworks, and serious volume expansion limit their further application in LIBs. Herein, we report a facile approach to obtain MXene-encapsulated porous Ni-naphthalene dicarboxylic acid (Ni-NDC) nanosheets by hybridizing ultrathin Ti3C2 MXene and three-dimensional (3D) Ni-NDC nanosheet aggregates. In the structure of Ni-NDC/MXene hybrids, the interlayer hydrogen-bond interaction between Ni-NDC and MXene can effectively increase the interlayer spacing and further inhibit the oxidation of pure MXene. Hence, the introduction of MXene (a conductive matrix) could further improve the conductivity of Ni-NDC, avoid self-agglomeration, and buffer the volume expansion of Ni-NDC nanosheets. Benefiting from the synergistic effects between Ni-NDC and MXene, Ni-NDC/MXene hybrid electrode exhibits a reversible discharge capacity (579.8 mA∙h∙g−1 at 100 mA∙g−1 after 100 cycles) and good long-term cycling performance (310 mA∙h∙g−1 at 1 A∙g−1 after 500 cycles).

Keywords

metal–organic frameworkMXenethree-dimensional porous intercalation structurelithium-ion battery

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Nano Research
Volume 16 Issue 2,
February 2023
Pages 2528-2535
DOI: 10.1007/s12274-022-5168-7
Cite this article:
Shi Y, Zhu G, Guo X, et al. Three-dimensional MXene-encapsulated porous Ni-NDC nanosheets as anodes for enhanced lithium-ion batteries. Nano Research, 2023, 16(2): 2528-2535. https://doi.org/10.1007/s12274-022-5168-7
Topics:
Lithium batteries

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Received: 07 September 2022
Revised: 05 October 2022
Accepted: 07 October 2022
Published: 15 December 2022
© Tsinghua University Press 2022
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