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Research Article

Two-dimensional CuO nanosheets-induced MOF composites and derivatives for dendrite-free zinc-ion batteries

Guoqiang Yuan1,§, Yang-Yi Liu1,2,§, Jun Xia3,§, Yichun Su1, Wenxian Wei1, YinBo Zhu3, Yang An1, HengAn Wu3, Qiang Xu4, Huan Pang1( )
School of Chemistry and Chemical Engineering, Yangzhou University, Yangzhou 225002, China
School of Electrical Engineering, Engineering Technology Research Center of Optoelectronic Technology Appliance, Tongling University, Tongling 244061, China
CAS Key Laboratory of Mechanical Behavior and Design of Materials, Department of Modern Mechanics, CAS Center for Excellence in Complex System Mechanics, University of Science and Technology of China, Hefei 230027, China
Department of Materials Science and Engineering, SUSTech Academy for Advanced Interdisciplinary Studies, Southern University of Science and Technology, Shenzhen 518055, China

§ Guoqiang Yuan, Yang-Yi Liu, and Jun Xia contributed equally to this work.

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Graphical Abstract

Inspired by electrostatic adsorption, carbon-coated Cu-Zn alloy nanosheets (CuZn@C NSs) were synthesized for the anodes of aqueous zinc-ion batteries (AZIBs). Due to the coexistence of Cu–Zn and Zn–N bonds, CuZn@C NSs anodes exhibit excellent zinc plating/peeling and cycle life in symmetric and half-cells. Low polarization, high capacity retention, and long cycle life were also achieved when CuZn@C NSs were used as anodes in asymmetric cells.

Abstract

Uncontrollable dendrite growth and side reactions resulting in short operating life and low Coulombic efficiency have severely hindered the further development of aqueous zinc-ion batteries (AZIBs). In this work, we designed to grow zeolitic imidazolate framework-8 (ZIF-8) uniformly on CuO nanosheets (NSs) and prepared carbon-coated CuZn alloy NSs (CuZn@C NSs) by calcination under H2/Ar atmosphere. As reflected by extended X-ray absorption fine structure (EXAFS), density functional theory (DFT), and in-situ Raman, the Cu–Zn and Zn–N bonds present in CuZn@C NSs act as zincophilic sites to uniformly absorb Zn ions and inhibit the formation of Zn dendrites. At the same time, CuZn@C NSs hinder the direct contact between zinc anode and electrolyte, preventing the occurrence of side reactions. More impressively, the symmetric cells constructed with CuZn@C NSs anodes exhibited excellent zinc plating/exfoliation performance and long life cycle at different current densities with low voltage hysteresis. In addition, low polarization, high capacity retention, and long cycle life over 1000 cycles at 5 A∙g−1 were achieved when CuZn@C NSs were used as anodes for CuZn@C/V2O5 full cells.

Keywords

two-dimensional CuO nanosheetmetal–organic frameworks (MOFs)-based compositescarbon-coated CuZn alloy nanosheetsdendrite-freezinc-ion battery

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Nano Research
Volume 16 Issue 5,
May 2023
Pages 6881-6889
DOI: 10.1007/s12274-023-5424-x
Cite this article:
Yuan G, Liu Y-Y, Xia J, et al. Two-dimensional CuO nanosheets-induced MOF composites and derivatives for dendrite-free zinc-ion batteries. Nano Research, 2023, 16(5): 6881-6889. https://doi.org/10.1007/s12274-023-5424-x
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Received: 23 October 2022
Revised: 24 November 2022
Accepted: 18 December 2022
Published: 03 February 2023
© Tsinghua University Press 2023
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