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Research Article

Photonic crystals constructed by isostructural metal-organic framework films

Zhihuan Li1, Jianxi Liu1( ), Haoze Wu1, Jiao Tang2, Zhongyang Li2, Yadong Xu1, Feng Zhou3, Weimin Liu1,3
State Key Laboratory of Solidification Processing, Center of Advanced Lubrication and Seal Materials, School of Materials Science and Engineering, Northwestern Polytechnical University, Xi’an 710072, China
Electronic Information School, Wuhan University, Wuhan 430072, China
State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, China
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Graphical Abstract

Isostructural metal-organic frameworks (MOFs)-based photonic crystals (PCs) are constructed by sequential spraying coating low refractive index (RI) layer of MOF and high RI layer of MOFs@nanoparticles. We demonstrated high detection sensitivity for chemical sensing on the PCs, which could be advanced by encapsulating different types of nanomaterials and designing wide-range color isostructural MOFs-based PCs.

Abstract

Metal-organic framework (MOF)-on-MOF structure allows stacking various types of MOFs with different lattice constants for molecule sieving or filtering. However, the multilayered MOFs-based optical devices have incoherent interference due to the lattice-mismatch at the interface and refractive index (RI) indifference. This paper reports isostructural MOFs-based photonic crystals (PCs) designed by stacking Bragg bilayers of lattice-matched MOFs thin films through a layer-by-layer assembly method. Colloidal nanoparticles (NPs) were homogenously encapsulated in some layers of the MOFs (HKUST-1@NPs) to tune their intrinsic RI during the spraying coating process. The isostructural MOFs-based PCs were constructed on a large scale by sequentially spraying coating the low RI layer of HKUST-1 and high RI layer of HKUST-1@NPs to form the desired number of Bragg bilayers. X-ray photoelectron spectroscopy (XPS) depth profiling proved the Bragg bilayers and the homogenous encapsulation of nanomaterials in certain layers of MOFs. Bandwidth of the PCs was tailored by the thickness and RI of the Bragg bilayers, which had a great consistent with finite difference time domain (FDTD) simulation. Importantly, reflectivity of the isostructural MOFs-based PCs was up to 96%. We demonstrated high detection sensitivity for chemical sensing on the PCs, which could be advanced by encapsulating different types of nanomaterials and designing wide-band isostructural MOFs-based PCs.

Keywords

metal-organic frameworks (MOFs)MOF on MOFliquid phase epitaxy (LPE)hybridphotonic crystals (PCs)specific sensing

Electronic Supplementary Material

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Nano Research
Volume 16 Issue 7,
July 2023
Pages 9569-9576
DOI: 10.1007/s12274-023-5505-5
Cite this article:
Li Z, Liu J, Wu H, et al. Photonic crystals constructed by isostructural metal-organic framework films. Nano Research, 2023, 16(7): 9569-9576. https://doi.org/10.1007/s12274-023-5505-5
Topics:
Chemical sensors DepositionOptical properties

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Received: 25 November 2022
Revised: 04 January 2023
Accepted: 08 January 2023
Published: 28 March 2023
© Tsinghua University Press 2023
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