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Research Article

Gap-surface-plasmon induced polarization photoresponse for MoS2-based photodetector

Qinghu Bai1,2,§, Xin Huang1,2,§( ), Yang Guo1,2, Shuo Du1,2, Chi Sun1,2, Leyong Hu1,2, Ruixuan Zheng1,2, Yang Yang1, Aizi Jin1, Junjie Li1,3, Changzhi Gu1,2( )
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China
School of Physical Sciences, CAS Key Laboratory of Vacuum Physics, University of Chinese Academy of Sciences, Beijing 100190, China
Songshan Lake Materials Laboratory, Dongguan 523808, China

§ Qinghu Bai and Xin Huang contributed equally to this work.

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Graphical Abstract

With the significant enhancement of electromagnetic field provided by the gap-surface-plasmon (GSP) of Au nanogroove, the MoS2 photodetector achieves a high photoresponsivity of 1.88 A/W and degree of linear polarization (DOLP) of 0.8 at the excitation wavelength of 633 nm.

Abstract

Polarization-sensitive photodetectors based on two-dimensional (2D) materials have shown more attractive application prospects compared to traditional thin-film photodetectors due to their atomic thickness, tunable bandgap, high mobility and strong light–matter interactions. Among them, 2D molybdenum disulfide (MoS2) has drawn numerous attentions in photodetection due to its wide spectral range, remarkable photoresponsivity and fast photo-switching rate. However, the isotropic crystal structure of MoS2 hampers its application in the polarization-sensitive detection, which is highly desired in military and civilian applications. In this paper, we demonstrated an integration of plasmonic nanocavity with monolayer MoS2 to achieve high photoresponsivity and polarization-sensitive photodetector. With the significant enhancement of electromagnetic field provided by the gap-surface-plasmon (GSP), we achieved a significant photoluminescence (PL) enhancement of 24-fold. Relying on the enhanced light absorption by our plasmonic nanocavity, which generally facilitates photo-generation of electron–hole pairs in MoS2, we achieved a high photoresponsivity of 1.88 A/W and degree of linear polarization (DOLP) of 0.8 at the excitation wavelength of 633 nm. Our work provides a feasible and universal solution to realize polarization-sensitive photodetector of MoS2 for high-performance and polarization-sensitive photodetectors.

Keywords

gap-surface-plasmonnanocavityMoS2photodetectorlinear polarization

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Nano Research
Volume 16 Issue 7,
July 2023
Pages 10272-10278
DOI: 10.1007/s12274-023-5724-9
Cite this article:
Bai Q, Huang X, Guo Y, et al. Gap-surface-plasmon induced polarization photoresponse for MoS2-based photodetector. Nano Research, 2023, 16(7): 10272-10278. https://doi.org/10.1007/s12274-023-5724-9
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Photodetectors

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Received: 10 February 2023
Revised: 26 March 2023
Accepted: 09 April 2023
Published: 26 June 2023
© Tsinghua University Press 2023
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