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Research Article

Magneto-electric integrated design strategy of NiCo@C composites for synergistic absorption and conversion in mid-high frequency microwaves

Yijie Liu1,2, Jintang Zhou1,2( ), Xiaoxuan He1,2, Lvtong Duan1,2, Yucheng Wang1,2, Zhenyu Cheng1,2, Zhengjun Yao1,2( )
College of Materials Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing 211100, China
Key Laboratory of Material Preparation and Protection for Harsh Environment (Nanjing University of Aeronautics and Astronautics), Ministry of Industry and Information Technology, Nanjing 211100, China
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Graphical Abstract

The morphology, composition, and defect states of NiCo@C materials are controlled by our chemical synthesis route. NiCo@C particles ultimately achieve synergistic absorption effects at low thickness (d < 3.5 mm) at middle frequencies (6–10 GHz) and high frequencies (10.5–18 GHz). Broadband absorption of electromagnetic waves and mid-high frequency band conversion are realized.

Abstract

Achieving synergistic absorption of electromagnetic waves (EMWs) in the mid-high frequency and absorption band conversion is an urgent problem. However, the present solution is usually a straightforward mixture of magnetic component-carbon component. Hereby, we optimize the magnetic properties and electrical relaxation response from a chemical synthesis perspective. Through integrated design, the contents of carbon components and multi-dimensional morphology are controlled by retaining strong magnetic properties. The morphology design and the construction of heterogeneous interfaces will boost the intense response of charge in the surrounding to enhance the polarization effect. The multi-dimensional structure and electromagnetic (EM) properties of the sample after optimized engineering have an extremely powerful absorption conversion effect on EMW energy. NiCo@C particles ultimately achieve synergistic absorption effects at low thickness (d < 3.5 mm) at middle frequencies (6–10 GHz) and high frequencies (10.5–18 GHz). Our work establishes a correlation mechanism between the physical and chemical properties of materials and EM parameters. It also provides insight into the synergistic absorption of EMWs in the mid-high frequency and absorption band conversion strategies.

Keywords

micro-nano compositesNiCo@Chollow structuremid-high frequency absorption

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Nano Research
Volume 17 Issue 4,
April 2024
Pages 2205-2215
DOI: 10.1007/s12274-023-6085-0
Cite this article:
Liu Y, Zhou J, He X, et al. Magneto-electric integrated design strategy of NiCo@C composites for synergistic absorption and conversion in mid-high frequency microwaves. Nano Research, 2024, 17(4): 2205-2215. https://doi.org/10.1007/s12274-023-6085-0
Topics:
Amorphous carbon

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Received: 14 July 2023
Revised: 04 August 2023
Accepted: 10 August 2023
Published: 11 October 2023
© Tsinghua University Press 2023
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