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Review Article

Interfacial engineering of the layered oxide cathode materials for sodium-ion battery

Quanqing Zhao1,§( ), Ruru Wang1,§, Ming Gao2, Faheem K. Butt3, Jianfeng Jia1( ), Haishun Wu1, Youqi Zhu4( )
Key Laboratory of Magnetic Molecules and Magnetic Information Materials of Ministry of Education, School of Chemistry and Materials Science, Shanxi Normal University, Taiyuan 030032, China
Metals and Chemistry Research Institute, China Academy of Railway Sciences Corporation Limited, Beijing 100081, China
Department of Physics, Division of Science and Technology, University of Education, Lahore 54770, Pakistan
Research Center of Materials Science, Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications, Beijing Institute of Technology, Beijing 100081, China

§ Quanqing Zhao and Ruru Wang contributed equally to this work.

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Graphical Abstract

The review discusses the mechanisms of bulk/surface degradation induced by oxygen loss, phase transition, crack, and electrolyte decomposition. The construction and stabilization mechanisms of interface via surface- and electrolyte-engineering are comprehensively evaluated.

Abstract

The layered metal oxides are reviewed as the hopeful cathode materials for high-performance sodium-ion batteries (SIBs) due to their large theoretical capacity, favorable two-dimensional (2D) ion diffusion channel, and simple manipuility. However, their cycling stability, rate capability, and thermal stability are still significantly concerned and highlighted before further practical application. The chemical, mechanical and electrochemical stability of the cathode–electrolyte interfaces upon cycling is of great significance. Herein, the unique structural and electrochemical properties of the layered oxide cathode materials for SIB are reviewed. The mechanism of bulk/surface degradation induced by oxygen evolution, phase transition, microcrack, and electrolyte decomposition is thoroughly understood. Furthermore, the interfacial engineering to construct stable interface through various effective methods is fully discussed. The future outlook and challenges for interfacial engineering in this filed are also summarized. This review should shed light on the rational design and construct of robust interface for applications of superior layered oxide cathodes in SIB and may suggest future research directions.

Keywords

interfacial engineeringsodium-ion batterylayered oxideelectrolyteinterface

Electronic Supplementary Material

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Nano Research
Volume 17 Issue 3,
March 2024
Pages 1441-1464
DOI: 10.1007/s12274-023-6133-9
Cite this article:
Zhao Q, Wang R, Gao M, et al. Interfacial engineering of the layered oxide cathode materials for sodium-ion battery. Nano Research, 2024, 17(3): 1441-1464. https://doi.org/10.1007/s12274-023-6133-9
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Secondary batteries

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Received: 21 July 2023
Revised: 24 August 2023
Accepted: 25 August 2023
Published: 09 October 2023
© Tsinghua University Press 2023
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