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Research Article

High MXene loading, nacre-inspired MXene/ANF electromagnetic interference shielding composite films with ultralong strain-to-failure and excellent Joule heating performance

Jiaen Wang1, Tianliang Song1, Wei Ming1, Moxi Yele1, Longfu Chen1, Hao Zhang1, Xiaojuan Zhang2( ), Benliang Liang1( ), Guangsheng Wang3
School of Physical Science and Engineering, Beijing Jiaotong University, Beijing 100044, China
College of Chemistry and Materials Engineering, Beijing Technology and Business University, Beijing 100048, China
Key Laboratory of Bio-Inspired Smart Interfacial Science and Technology of Ministry of Education, School of Chemistry, Beihang University, Beijing 100191, China
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Graphical Abstract

Even though the functional filler MXene contents are as high as 60 wt.% and 70 wt.%, the strain-to-failure of the films could reach astonishing values of 18.34% ± 1.86% and 14.43% ± 1.26%, respectively, so the films can also withstand double folding and vigorous rubbing without damage, which could better adapt to a harsh application environment, at the same time, the corresponding electromagnetic interference (EMI) shielding effectiveness (SE) values could reach 45 and 52.15 dB. Inspired by nacre, the three-dimensional (3D) interconnected aramid nanofiber (ANF) networks between adjacent layered MXene give MXene/ANF composite films toughness and functional unity in the presence of high-functional fillers, which means this work provides a convenient way to prepare other high functional filler composite films with excellent mechanical performance.

Abstract

The high power density and intelligence of next-generation flexible electronic devices bring many challenges to fabricate flexible composite films with electromagnetic interference (EMI) shielding effectiveness (SE) property and excellent toughness via a simple method. Herein, inspired by the layered structure and biopolymer matrix networks in natural nacre, nacre-like layered Ti3C2TX (MXene)/aramid nanofiber (ANF) films were fabricated through sol-gel, vacuum-assisted filtration, and hot-pressing. Three-dimensional (3D) interconnected aramid nanofibers networks between adjacent layered MXene result in an ultralong strain-to-failure of the film. Even though the functional filler MXene contents are as high as 60 wt.% and 70 wt.%, the strain-to-failure of the films could reach astonishing values of 18.34% ± 1.86% and 14.43% ± 1.26%, respectively. And the tensile strength could maintain about 85 MPa. Excitingly, with such a high filler, the film can also withstand double folding and vigorous rubbing without damage, which could better adapt to a harsh application environment. The result means that this work provides a convenient way to prepare other high functional filler composite films with excellent mechanical performance. The EMI SE values could reach 45 and 52.15 dB at 60 wt.% and 70 wt.% MXene in 8.2–12.4 GHz. Meanwhile, the films have prominent Joule heating properties, high sensitivity (< 15 s), small voltage operation (0.5 V), and high operation constancy (1300 s). Therefore, nacre-inspired MXene/ANF composite films in this work have ability to apply in many areas including communication technology, military, and aerospace.

Keywords

bioinspiredaramid nanofiber networksultralong strain-to-failuretoughening mechanismelectromagnetic interference shielding

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Nano Research
Volume 17 Issue 3,
March 2024
Pages 2061-2069
DOI: 10.1007/s12274-023-6232-y
Cite this article:
Wang J, Song T, Ming W, et al. High MXene loading, nacre-inspired MXene/ANF electromagnetic interference shielding composite films with ultralong strain-to-failure and excellent Joule heating performance. Nano Research, 2024, 17(3): 2061-2069. https://doi.org/10.1007/s12274-023-6232-y
Topics:
NanofibersNanosheetsNanostructuresThin films
Part of a topical collection:
EM Wave Functional Materials

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Received: 05 September 2023
Revised: 21 September 2023
Accepted: 23 September 2023
Published: 18 November 2023
© Tsinghua University Press 2023
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