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Research Article

Flexible mille-feuille structure electromagnetic interference shielding film with excellent thermal conductivity and Joule heating

Dingwen Yin1,2, Huijuan Xiu1,2( ), Simin Wang1,2, Yanfei Pan3( ), Na Li1,2, Rui Cheng1,2, Shaoyan Huang1,2, Sha Fan1,2, Jinbao Li1,2( )
College of Bioresources Chemical & Materials Engineering, Shaanxi University of Science & Technology, Xi'an 710021, China
National Demonstration Center for Experimental Light Chemistry Engineering Education, Shaanxi Provincial Key Laboratory of Papermaking Technology and Specialty Paper Development, Xi'an 710021, China
College of Material Science and Art Design, Inner Mongolia Agricultural University, Hohhot 010018, China
Show Author Information

Graphical Abstract

Flexible mille-feuille structure composite films were fabricated via the layer-by-layer self-assembly and hot-pressing strategy of the TEMPO-oxidized cellulose nanofibrils/silver nanoparticles (TOCNFs/AgNPs) and graphene nanoplates (GNPs). The composite film possessed superb electromagnetic interference (EMI) shielding (98.05 dB), excellent thermal conductivity (18.82 W/(m·K)) and outstanding Joule heating.

Abstract

The intelligent electronic devices have urgent demands for electromagnetic interference (EMI) shielding films with excellent heat dissipation capability. However, it is challenging to obtain excellent EMI shielding and thermal conductivity performances simultaneously. Herein, inspired by mille-feuille structure, the multifunctional EMI shielding films developed by a layer-by-layer self-assembly and hot-pressing strategy. The ingenious introduction of silver nanoparticles (AgNPs) with large specific surface area and highly conductive into the network formed by TEMPO-oxidized cellulose nanofibrils (TOCNFs) with large aspect ratio to form the TOCNFs/AgNPs. And the graphene nanoplates (GNPs) with high conductivity loss distributed alternately with TOCNFs/AgNPs to construct mille-feuille structure, which had highly efficient conductive network, complete thermally conduction pathway and rich heterogeneous interfaces. Consequently, the designed films presented high electrical conductivity of 8520 S/cm, superb EMI effectiveness (SE) of 98.05 dB, and excellent thermal conductivity of 18.82 W/(m·K). Furthermore, the films possessed outstanding Joule heating performances with low voltages, including high heating temperature (100 °C), fast response time (< 20 s), and impressive heating stability and reliability. Thus, such high-performance EMI shielding films with fascinating thermal conductivity and Joule heating performances have substantial application in flexible electronics, electromagnetic waves shielding and thermal management.

Keywords

TEMPO-oxidized cellulose nanofibrils/silver nanoparticles (TOCNFs/AgNPs)mille-feuille structureelectromagnetic interference shieldingthermal conductivityJoule heating

Electronic Supplementary Material

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12274_2023_6387_MOESM1_ESM.pdf (3.6 MB)

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Nano Research
Volume 17 Issue 5,
May 2024
Pages 4544-4554
DOI: 10.1007/s12274-023-6387-2
Cite this article:
Yin D, Xiu H, Wang S, et al. Flexible mille-feuille structure electromagnetic interference shielding film with excellent thermal conductivity and Joule heating. Nano Research, 2024, 17(5): 4544-4554. https://doi.org/10.1007/s12274-023-6387-2
Topics:
GrapheneNanocompositesNanofibersSilver nanoparticles

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Received: 09 October 2023
Revised: 21 November 2023
Accepted: 01 December 2023
Published: 12 January 2024
© Tsinghua University Press 2023
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