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Research Article

Construction of flower-like MoS2 decorated on Cu doped CoZn-ZIF derived N-doped carbon as superior microwave absorber

Yun Han1,§, Di Lan2,§, Mengjun Han1,§, Zihao Xia1, Jiaxiao Zou1, Zirui Jia1( )
College of Chemistry and Chemical Engineering, Qingdao University, Qingdao 266071, China
School of Materials Science and Engineering, Hubei University of Automotive Technology, Shiyan 442002, China

§ Yun Han, Di Lan, and Mengjun Han contributed equally to this work.

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Graphical Abstract

Cu/Co-NC/MoS2 composites with unique flower-like morphology was prepared to optimize the electromagnetic synergy strategy between components and to modulate the complex dielectric parameters of the materials, thus exhibiting outstanding microwave absorption properties.

Abstract

The rational design of composition nanostructures and morphologies of the carbon-based composites materials has a significant potential for tuning electromagnetic parameters and thereby improving their performance as electromagnetic wave (EMW) absorbers. In this work, the flower-like Cu/Co-NC/MoS2 (NC = N-doped carbon skeleton) composites were successfully prepared by employing CuCoZn-ZIF (ZIF = zeolitic imidazolate framework) as precursor with subsequent annealing and hydrothermal technique. The unique flower-like morphology and electromagnetic synergy strategy between components enable the as-obtained Cu/Co-NC/MoS2 composites to exhibit outstanding microwave absorption properties. Accordingly, the minimum reflection loss of Cu/Co-NC/MoS2 reaches −54.36 dB at 2.7 mm. When the thickness reduces to 2.2 mm, the maximum effective absorption bandwidth can be achieved as large as 6.72 GHz. This research develops useful ideas for optimizing multicomponent microwave absorbing materials.

Keywords

MoS2microwave absorptionflower-like morphologyternary metal-organic frameworks (MOFs)

Electronic Supplementary Material

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Nano Research
Volume 17 Issue 9,
September 2024
Pages 8250-8260
DOI: 10.1007/s12274-024-6859-z
Cite this article:
Han Y, Lan D, Han M, et al. Construction of flower-like MoS2 decorated on Cu doped CoZn-ZIF derived N-doped carbon as superior microwave absorber. Nano Research, 2024, 17(9): 8250-8260. https://doi.org/10.1007/s12274-024-6859-z
Topics:
NanocompositesNanostructured materialsNanostructuresOrganic frameworks

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Received: 06 June 2024
Revised: 26 June 2024
Accepted: 02 July 2024
Published: 23 July 2024
© Tsinghua University Press 2024
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