AI Chat Paper
Note: Please note that the following content is generated by AMiner AI. SciOpen does not take any responsibility related to this content.
{{lang === 'zh_CN' ? '文章概述' : 'Summary'}}
{{lang === 'en_US' ? '中' : 'Eng'}}
Chat more with AI
Powered by AMiner. Clicking this button will take you away from SciOpen.
Home Journal of Advanced Ceramics Article
PDF (2.2 MB)
Cite
EndNote(RIS) BibTeX
Collect
Submit Manuscript AI Chat Paper
Show Outline
Outline
Show full outline
Hide outline
Outline
Show full outline
Hide outline
Research Article | Open Access

ZrB2 particles reinforced glass coating for oxidation protection of carbon/carbon composites

Cuiyan LI( ), Guibiao LI, Haibo OUYANG, Jing LU
School of Materials Science & Engineering, Shaanxi University of Science & Technology, Xi’an 710021, China
Show Author Information

Abstract

A dense ZrB2 particles reinforced glass (ZrB2/SiO2) coating was prepared on the SiC coated carbon/carbon composites by a facile sol-dipping approach. The prepared ZrB2/SiO2 coating could protect the composites from being oxidized for 160 h at 1773 K with a weight loss of 6.9 mg/cm2. The flexural strength retention ratio of the ZrB2/SiO2 coated composites is 87% after oxidation for 160 h at 1773 K. The continuous SiO2 glass layer embedded with the submicron ZrSiO4 particles was formed during oxidation. This was helpful to lower the diffusion rate of oxygen and improve the stability of SiO2 glass film, thus improving the oxidation resistance of the coated samples. After thermal cycles between 1773 K and room temperature for 15 times, penetrated cracks formed in the coating. The weight loss of the ZrB2/SiO2 coated sample presented linear relationship, and the final weight loss per unit area was 6.35 mg/cm2. The generation of the penetrative cracks and the debonded coating interface resulted in the failure of the ZrB2/SiO2 coating.

Keywords

ZrB2/SiO2 coatingsilica soldippingoxidation resistance

References

[1]
B Xu, R He, C Hong, et al. Ablation behavior and mechanism of double-layer ZrB2-based ceramic coating for lightweight carbon-bonded carbon fiber composites under oxyacetylene flame at elevate temperature. J Alloys Compd 2017, 702: 551-560.
Crossref Google Scholar
[2]
A Purwar, B Basu. Thermo-structural design of ZrB2-SiC-based thermal protection system for hypersonic space vehicles. J Am Ceram Soc 2017, 100: 1618-1633.
Crossref Google Scholar
[3]
S Zhou, Y Qi, P Wang, et al. A ZrB2-SiC/SiC oxidation protective dual-layer coating for carbon/carbon composites. Adv Appl Ceram 2017, 116: 462-467.
Crossref Google Scholar
[4]
X Yang, W Li, S Wang, et al. ZrB2 coating for the oxidation protection of carbon fiber reinforced silicon carbide matrix composites. Vacuum 2013, 96: 63-68.
Crossref Google Scholar
[5]
Y Niu, Z Wang, J Zhao, et al. Comparison of ZrB2-MoSi2 composite coatings fabricated by atmospheric and vacuum plasma spray processes. J Therm Spray Tech 2017, 26: 100-107.
Crossref Google Scholar
[6]
Q-G Fu, J-Y Jing, B-Y Tan, et al. Nanowire-toughened transition layer to improve the oxidation resistance of SiC-MoSi2-ZrB2 coating for C/C composites. Corros Sci 2016, 111: 259-266.
Crossref Google Scholar
[7]
L Silvestroni, D Sciti. Densification of ZrB2-TaSi2 and HfB2-TaSi2 ultra-high-temperature ceramic composites. J Am Ceram Soc 2011, 94: 1920-1930.
Crossref Google Scholar
[8]
X-Y Yao, H-J Li, Y-L Zhang, et al. A SiC/ZrB2-SiC/SiC oxidation resistance multilayer coating for carbon/carbon composites. Corros Sci 2012, 57: 148-153.
Crossref Google Scholar
[9]
K Li, M Hu, Dynamic oxidation resistance and residual mechanical strength of ZrB2-CrSi2-SiC-Si/SiC coated C/C composites. Ceram Int 2017, 43: 4880-4887.
Crossref Google Scholar
[10]
T Feng, H-J Li, X-H Shi, et al. Oxidation and ablation resistance of ZrB2-SiC-Si/B-modified SiC coating for carbon/carbon composites. Corros Sci 2013, 67: 292-297.
Crossref Google Scholar
[11]
SS Hwang, AL Vasiliev, NP Padture. Improved processing and oxidation-resistance of ZrB2 ultra-high temperature ceramics containing SiC nanodispersoids. Mat Sci Eng A 2007, 464: 216-224.
Crossref Google Scholar
[12]
X Yao, H Li, Y Zhang, et al. A SiC-Si-ZrB2 multiphase oxidation protective ceramic coating for SiC-coated carbon/ carbon composites. Ceram Int 2012, 38: 2095-2100.
Crossref Google Scholar
[13]
J Pourasad, N Ehsani, Z Valefi. Oxidation resistance of a SiC-ZrB2 coating prepared by a novel pack cementation on SiC-coated graphite. J Mater Sci 2017, 52: 1639-1646.
Crossref Google Scholar
[14]
L Li, H Li, X Yin, et al. Microstructure evolution of SiC-ZrB2-ZrC coating on C/C composites at 1773 K under different oxygen partial pressures. J Alloys Compd 2016, 687: 470-479.
Crossref Google Scholar
[15]
L Wang, Q-G Fu, F-L Zhao. A novel gradient SiC-ZrB2- MoSi2 coating for SiC coated C/C composites by supersonic plasma spraying. Surf Coat Technol 2017, 313: 63-72.
Crossref Google Scholar
[16]
Y Niu, H Wang, H Li, et al. Dense ZrB2-MoSi2 composite coating fabricated by low pressure plasma spray (LPPS). Ceram Int 2013, 39: 9773-9777.
Crossref Google Scholar
[17]
X Yang, W Li, S Wang, et al. ZrB2/SiC as a protective coating for C/SiC composites: Effect of high temperature oxidation on mechanical properties and anti-ablation property. Composites Part B 2013, 45: 1391-1396.
Crossref Google Scholar
[18]
H Ouyang, C Li, J Huang, et al. Self-healing ZrB2-SiO2 oxidation resistance coating for SiC coated carbon/carbon composites. Corros Sci 2016, 110: 265-272.
Crossref Google Scholar
[19]
X Yao, S Tan, Z Huang, et al. Dispersion of talc particles in a silica sol. Mater Lett 2005, 59: 100-104.
Crossref Google Scholar
[20]
M Tomas, H Amaveda, LA Angurel, et al. Effect of silica sol on the dispersion-gelation process of concentrated silica suspensions for fibre-reinforced ceramic composites. J Eur Ceram Soc 2013, 33: 727-736.
Crossref Google Scholar
[21]
X Zhu, D Jiang, S Tan, et al. Dispersion properties of alumina powders in silica sol. J Eur Ceram Soc 2001, 21: 2879-2885.
Crossref Google Scholar
[22]
I Santana, A Pepe, E Jimenez-Pique, et al. Corrosion protection of carbon steel by silica-based hybrid coatings containing cerium salts: Effect of silica nanoparticle content. Surf Coat Technol 2015, 265: 106-116.
Crossref Google Scholar
[23]
Q Ma, L Cai. Fabrication and oxidation resistance of mullite/yttrium silicate multilayer coatings on C/SiC composites. J Adv Ceram 2017, 6: 360-367.
Crossref Google Scholar
[24]
Q Ma, L Cai. Fabrication of Y2Si2O7 coating and its oxidation protection for C/SiC composites. Trans Nonferrous Met Soc China 2017, 27: 390-396.
Crossref Google Scholar
[25]
Q-G Fu, H-J Li, X-H Shi, et al. Silicon carbide coating to protect carbon/carbon composites against oxidation. Scripta Mater 2005, 52: 923-927.
Crossref Google Scholar
[26]
L Wang, Q Fu, F Zhao, A novel gradient SiC-ZrB2-MoSi2 coating for SiC coated C/C composites by supersonic plasma spraying. Surf Coat Technol 2017, 313: 63-72.
Crossref Google Scholar
[27]
X Yang, W Li, S Wang, et al. Ablative property of ZrC-SiC multilayer coating for PIP-C/SiC composites under oxy-acetylene torch. Ceram Int 2012, 38: 2893-2897.
Crossref Google Scholar
[28]
J Pourasad, N Ehsani. In-situ synthesis of SiC-ZrB2 coating by a novel pack cementation technique to protect graphite against oxidation. J Alloys Compd 2017, 690: 692-698.
Crossref Google Scholar
[29]
H Jin, S Meng, X Zhang, et al. Oxidation of ZrB2-SiC-graphite composites under low oxygen partial pressures of 500 and 1500 Pa at 1800 ℃. J Am Ceram Soc 2016, 99: 2474-2480.
Crossref Google Scholar
[30]
G Ouyang, PK Ray, MJ Kramer, et al. High-temperature oxidation of ZrB2-SiC-AlN composites at 1600 ℃. J Am Ceram Soc 2016, 99: 808-813.
Crossref Google Scholar
[31]
X Ren, H Li, Y Chu, et al. Preparation of oxidation protective ZrB2-SiC coating by in-situ reaction method on SiC-coated carbon/carbon composites. Surf Coat Technol 2014, 247: 61-67.
Crossref Google Scholar
[32]
Y Zhang, H Hu, P Zhang, et al. SiC/ZrB2-SiC-ZrC multilayer coating for carbon/carbon composites against ablation. Surf Coat Technol 2016, 300: 1-9.
Crossref Google Scholar
[33]
X Fan, W Huang, H Liu, et al. Bond stability and oxidation resistance of BSAS-based coating on C/SiC composites. Surf Coat Technol 2017, 309: 35-46.
Crossref Google Scholar
Journal of Advanced Ceramics
Volume 8 Issue 1,
March 2019
Pages 102-111
DOI: 10.1007/s40145-018-0298-9
Cite this article:
LI C, LI G, OUYANG H, et al. ZrB2 particles reinforced glass coating for oxidation protection of carbon/carbon composites. Journal of Advanced Ceramics, 2019, 8(1): 102-111. https://doi.org/10.1007/s40145-018-0298-9

955

Views

52

Downloads

55

Crossref

N/A

Web of Science

57

Scopus

0

CSCD

Altmetrics
Received: 06 June 2018
Revised: 30 September 2018
Accepted: 01 October 2018
Published: 13 March 2019
© The author(s) 2019

Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made.

The images or other third party material in this article are included in the article’s Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder.

To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/.
Return