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Review | Open Access

Si-based polymer-derived ceramics for energy conversion and storage

Qingbo WENa,†, Fangmu QUc,†, Zhaoju YUb( ), Magdalena GRACZYK-ZAJACc,d( ), Xiang XIONGa, Ralf RIEDELc
State Key Laboratory of Powder Metallurgy, Central South University, Changsha 410083, China
College of Materials, Key Laboratory of High-Performance Ceramic Fibers (Xiamen University), Ministry of Education, Xiamen 361005, China
Technische Universität Darmstadt, Institut für Materialwissenschaft, Otto-Berndt-Straße 3, D-64287, Darmstadt, Germany
EnBW Energie Baden-Württemberg AG, Durlacher Allee 93, 76131 Karlsruhe, Germany

† Qingbo Wen and Fangmu Qu contributed equally to this work.

Show Author Information
An erratum to this article is available online at:
https://doi.org/10.1007/s40145-022-0600-8

Graphical Abstract

Abstract

Since the 1960s, a new class of Si-based advanced ceramics called polymer-derived ceramics (PDCs) has been widely reported because of their unique capabilities to produce various ceramic materials (e.g., ceramic fibers, ceramic matrix composites, foams, films, and coatings) and their versatile applications. Particularly, due to their promising structural and functional properties for energy conversion and storage, the applications of PDCs in these fields have attracted much attention in recent years. This review highlights the recent progress in the PDC field with the focus on energy conversion and storage applications. Firstly, a brief introduction of the Si-based polymer-derived ceramics in terms of synthesis, processing, and microstructure characterization is provided, followed by a summary of PDCs used in energy conversion systems (mainly in gas turbine engines), including fundamentals and material issues, ceramic matrix composites, ceramic fibers, thermal and environmental barrier coatings, as well as high-temperature sensors. Subsequently, applications of PDCs in the field of energy storage are reviewed with a strong focus on anode materials for lithium and sodium ion batteries. The possible applications of the PDCs in Li-S batteries, supercapacitors, and fuel cells are discussed as well. Finally, a summary of the reported applications and perspectives for future research with PDCs are presented.

Keywords

polymer-derived ceramics (PDCs)high-temperature resistancestructural propertieselectrochemical propertiesmicrostructure

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Journal of Advanced Ceramics
Volume 11 Issue 2,
February 2022
Pages 197-246
DOI: 10.1007/s40145-021-0562-2
Cite this article:
WEN Q, QU F, YU Z, et al. Si-based polymer-derived ceramics for energy conversion and storage. Journal of Advanced Ceramics, 2022, 11(2): 197-246. https://doi.org/10.1007/s40145-021-0562-2

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Received: 30 September 2021
Revised: 05 December 2021
Accepted: 07 December 2021
Published: 11 January 2022
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