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Research Article | Open Access

Tribological properties of polyimide composites reinforced with fibers rubbing against Al2O3

Huimin QI1,2Ga ZHANG2,3Zhiqin ZHENG4Jiaxin YU1( )Chao HU3
Key Laboratory of Testing Technology for Manufacturing Process in Ministry of Education, State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology, Mianyang 621010, China
State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences, Lanzhou 730000, China
Qingdao Center of Resource Chemistry & New Materials, Qingdao 266071, China
Fundamental Science on Nuclear Wastes and Environmental Safety Laboratory, Southwest University of Science and Technology, Mianyang 621010, China
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Abstract

Reinforcing fillers are of great importance in tribological performance and tribofilm formation of polymeric composites. In this study, the tribological properties of aramid particle (AP) and short carbon fiber (SCF) reinforced polyimide (PI) composites were added to hexagonal boron nitride (h-BN), and silica (SiO2) nanoparticles sliding against alumina were comprehensively investigated. When sliding occurred with AP-reinforced PI composites, the tribological properties were not closely depended on the pressure × velocity (p × v) factors and the nanoparticles. The interactions between AP and its counterpart could not induce tribo-sintering of the transferred wear debris. As such, the tribofilm seemed to be in a viscous state, leading to higher friction and wear. However, the inclusion of hard SCF into the PI matrix changed the interfacial interactions with alumina. A robust tribofilm consisting of a high fraction of silica was generated when the SCF-reinforced PI was added to the SiO2 nanoparticles. It exhibited a high load-carrying capability and was easily sheared. This caused a significant decrease in the friction and wear of the PI composite at 8 MPa·1m/s. Moreover, due to their high melting point, few h-BN nanoparticles were observed in the tribofilm of the SCF-reinforced PI when hexagonal boron nitride was added.

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Friction
Pages 301-314
Cite this article:
QI H, ZHANG G, ZHENG Z, et al. Tribological properties of polyimide composites reinforced with fibers rubbing against Al2O3. Friction, 2021, 9(2): 301-314. https://doi.org/10.1007/s40544-019-0339-6

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Received: 27 May 2019
Revised: 08 October 2019
Accepted: 28 October 2019
Published: 09 May 2020
© The author(s) 2019

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