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Research paper | Open Access

Ultra-slim electrostrains with superior temperature-stability in lead-free sodium niobate-based ferroelectric perovskite

Ruiyi Jinga, Qingyuan Hua, Leiyang Zhanga, Yuan Sunb, Jiagang Wuc, D.O. Alikind, V. Ya Shurd, Xiaoyong Weia, Hongliang Due, Yunfei Changb( ), Li Jina( )
Electronic Materials Research Laboratory, Key Laboratory of the Ministry of Education & International Center for Dielectric Research, School of Electronic Science and Engineering, Xi'an Jiaotong University, Xi'an, 710049, China
Functional Materials and Acousto-Optic Instruments Institute, School of Instrumentation Science and Engineering, Harbin Institute of Technology, Harbin, 150080, China
Department of Materials Science, Sichuan University, Chengdu, 610065, China
School of Natural Sciences and Mathematics, Ural Federal University, Ekaterinburg, 620000, Russia
Multifunctional Electronic Ceramics Laboratory, College of Engineering, Xi'an International University, Xi'an, 710077, China

Peer review under responsibility of The Chinese Ceramic Society.

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Graphical Abstract

Abstract

Large electrostrains with high temperature stability and low hysteresis are essential for applications in high-precision actuator devices. However, achieving simultaneously all three of the aforementioned features in ferroelectric ceramics remains a considerable challenge. In this work, we firstly report a high unipolar electrostrain (0.12% at 60 kV/cm) in (1–x)NaNbO3-x[(Ba0.85Ca0.15)(Zr0.1Ti0.9)O3] (NN-xBCZT) ferroelectric polycrystalline ceramics with excellent thermal stability (variation less than 10% in the temperature range of 30–160 ℃) and ultra-low hysteresis (< 6%). Secondly, the high-field electrostrain response is dominated by the intrinsic electrostrictive effect, which may account for more than 80% of the electrostrain. Furthermore, due to the thermal stability of the polarization in the pure tetragonal phase, the large electrostrain demonstrates extraordinarily high stability from room temperature to 140 ℃. Finally, in-situ piezoelectric force microscopy reveals ultra-highly stable domain structures, which also guarantee the thermal stability of the electrostrain in (NN-xBCZT ferroelectrics ceramics. This study not only clarifies the origin of thermally stable electrostrain in NN-xBCZT ferroelectric perovskite in terms of electrostrictive effect, but also provides ideas for developing applicable ferroelectric ceramic materials used in actuator devices with excellent thermal stability.

Keywords

PolarizationElectrostrainNaNbO3Electrostriction

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Journal of Materiomics
Volume 8 Issue 6,
November 2022
Pages 1230-1238
DOI: 10.1016/j.jmat.2022.05.002
Cite this article:
Jing R, Hu Q, Zhang L, et al. Ultra-slim electrostrains with superior temperature-stability in lead-free sodium niobate-based ferroelectric perovskite. Journal of Materiomics, 2022, 8(6): 1230-1238. https://doi.org/10.1016/j.jmat.2022.05.002

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Received: 27 March 2022
Revised: 05 May 2022
Accepted: 11 May 2022
Published: 17 May 2022
© 2022 The Chinese Ceramic Society.

This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).
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