Enhanced energy storage properties and good stability of novel (1–x)Na0.5Bi0.5TiO3–xCa(Mg1/3Nb2/3)O3 relaxor ferroelectric ceramics prepared by chemical modification

Ying Zhang; Meng-Han Yan; Zhi-Fei Zhang; Hai-Rui Bai; Peng Li; Wei-Fang Han; Ji-Gong Hao; Wei Li; Yu-Chao Li; Chun-Ming Wang; Peng Fu

doi:10.1016/j.jmat.2023.09.009

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Research Article | Open Access

Enhanced energy storage properties and good stability of novel (1–x)Na_0.5Bi_0.5TiO₃–xCa(Mg_1/3Nb_2/3)O₃ relaxor ferroelectric ceramics prepared by chemical modification

Ying Zhang^{^a}, Meng-Han Yan^{^a}, Zhi-Fei Zhang^{^a}, Hai-Rui Bai^{^b}(

), Peng Li^{^a}, Wei-Fang Han^{^a}, Ji-Gong Hao^{^a}, Wei Li^{^a}(

), Yu-Chao Li^{^a}, Chun-Ming Wang^{^c}, Peng Fu^{^a^,^c}(

)

School of Materials Science and Engineering, Liaocheng University, Liaocheng, 252059, China

Shandong Laboratory of Yantai Advanced Materials and Green Manufacturing, 300 Changjiang Road, Yantai, 264006, China

School of Physics, Shandong University, Jinan, 250100, China

Peer review under responsibility of The Chinese Ceramic Society.

Show Author Information

Graphical Abstract

Abstract

The increase in energy consumption and its collateral damage on the environment has encouraged the development of environment-friendly ceramic materials with good energy storage properties. In this work, (1–x)Na_0.5Bi_0.5TiO₃-xCa(Mg_1/3Nb_2/3)O₃ ceramics were synthesized by the solid-state reaction method. The 0.88Na_0.5Bi_0.5TiO₃-0.12Ca(Mg_1/3Nb_2/3)O₃ ceramic exhibited a high recoverable energy storage density of 8.1 J/cm³ and energy storage efficiency of 82.4% at 550 kV/cm. The introduction of Ca(Mg_1/3Nb_2/3)O₃ reduced the grain size and increased the band gap, thereby enhancing the breakdown field strength of the ceramic materials. The method also resulted in good temperature stability (20–140 ℃), frequency stability (1–200 Hz), and fatigue stability over 10⁶ cycles. In addition, an ultrahigh power density of 187 MW/cm³ and a fast charge-discharge rate (t_0.9 = 57.2 ns) can be obtained simultaneously. Finite element method analysis revealed that the decrease of grain size was beneficial to the increase of breakdown field strength. Therefore, the 0.88Na_0.5Bi_0.5TiO₃-0.12Ca(Mg_1/3Nb_2/3)O₃ ceramics resulted in high energy storage properties with good stability and were promising environment-friendly materials for advanced pulsed power systems applications.

Keywords

Stability Relaxor ferroelectrics Energy storage properties Breakdown field strength (1–x)Na_0.5Bi_0.5TiO₃-xCa(Mg_1/3Nb_2/3)O₃ ceramics

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Journal of Materiomics

Volume 10 Issue 4,
July 2024

Pages 770-782

DOI: 10.1016/j.jmat.2023.09.009

Cite this article:

Zhang Y, Yan M-H, Zhang Z-F, et al. Enhanced energy storage properties and good stability of novel (1–x)Na_0.5Bi_0.5TiO₃–xCa(Mg_1/3Nb_2/3)O₃ relaxor ferroelectric ceramics prepared by chemical modification. Journal of Materiomics, 2024, 10(4): 770-782. https://doi.org/10.1016/j.jmat.2023.09.009

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Received: 20 June 2023

Revised: 28 August 2023

Accepted: 07 September 2023

Published: 12 October 2023

This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).