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Research Article | Open Access

Developing high photocatalytic antibacterial Zn electrodeposited coatings through Schottky junction with Fe3+-doped alkalized g-C3N4 photocatalysts

Ying Gaoa,b,c,d, Xiaofan Zhaia,c,d( ), Yuxin Zhange, Fang Guana,c,d, Nazhen Liua,c,d, Xiutong Wanga,c,d, Jie Zhanga,c,d, Baorong Houa,c,d, Jizhou Duana,c,d( )
Key Laboratory of Marine Environmental Corrosion and Bio-Fouling, Institute of Oceanology, Chinese Academy of Sciences, Qingdao, 266071, China
University of Chinese Academy of Sciences, Beijing, 100049, China
Open Studio for Marine Corrosion and Protection, Pilot National Laboratory for Marine Science and Technology (Qingdao), Qingdao, 266071, China
Center for Ocean Mega-Science, Chinese Academy of Sciences, Qingdao, 266071, China
College of Materials Science and Engineering, Chongqing University, Chongqing, 400044, China
Show Author Information

Abstract

Pure Zn coatings easily lose their protective performance after biofouling because they have no antibacterial effect under visible light. In this study, we fabricate a new antibacterial Zn composite coating using electrodeposition to couple Fe3+-doped alkalized g-C3N4 (AKCN-Fe) into an existing Zn coating and show that the AKCN-Fe enhances antibacterial property of the Zn coating under visible light. We attribute this enhancement to the high photocatalytic performance, high loading content, and good dispersion of AKCN-Fe. In addition, the photocatalytic antibacterial mechanism of the composite coating is supported by scavenger experiments and electron paramagnetic resonance (EPR) measurements, suggesting that superoxide () and hydroxyl radical (·OH) play main and secondary roles, respectively.

Keywords

Electrodepositiong-C3N4Zn coatingPhotocatalytic antibacterial mechanism

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Nano Materials Science
Volume 5 Issue 2,
June 2023
Pages 177-188
DOI: 10.1016/j.nanoms.2022.01.004
Cite this article:
Gao Y, Zhai X, Zhang Y, et al. Developing high photocatalytic antibacterial Zn electrodeposited coatings through Schottky junction with Fe3+-doped alkalized g-C3N4 photocatalysts. Nano Materials Science, 2023, 5(2): 177-188. https://doi.org/10.1016/j.nanoms.2022.01.004

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Received: 12 November 2021
Accepted: 31 December 2021
Published: 14 February 2022
© 2023 Chongqing University.

This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).
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