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Paper | Open Access

Cooling rate calibration and mapping of ultra-short pulsed laser modifications in fused silica by Raman and Brillouin spectroscopy

Michael Bergler1,2,3, Kristian Cvecek1,3, Ferdinand Werr2, Martin Brehl2, Dominique De Ligny2, Michael Schmidt1,3
Friedrich-Alexander-Universität Erlangen-Nürnberg, Institute of Photonic Technologies, Erlangen, Germany
Friedrich-Alexander-Universität Erlangen-Nürnberg, Institute of Glass and Ceramics, Erlangen, Germany
Friedrich-Alexander-Universität Erlangen-Nürnberg, SAOT – Erlangen Graduate School in Advanced Optical Technologies, Erlangen, Germany
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Abstract

This paper focuses on the preparation of a new extended set of calibrations of cooling rate (fictive temperature) in fused silica determined by inelastic light scattering and its subsequent use to characterize the local cooling rate distribution in ultra-short pulsed (USP) laser modification. In order to determine the thermal history (e.g. cooling rate and fictive temperature) of fused silica, high-resolution inelastic light-scattering experiments (Raman and Brillouin spectroscopy) were investigated. Calibrations were performed and compared to the existing literature to quantify structural changes due to a change of fictive temperature. Compared to existing calibrations, this paper provides an extension to lower and higher cooling rates. Using this new set of calibrations, we characterized a USP laser modification in fused silica and calculated the local fictive temperature distribution. An equation relating the fictive temperature (Tf) to cooling rates is given. A maximum cooling rate of 3000 K min−1 in the glass transition region around 1200 ℃ was deduced from the Raman analysis. The Brillouin observations are sensitive to both the thermal history and the residual stress. By comparing the Raman and Brillouin observations, we extracted the local residual stress distribution with high spatial resolution. For the first time, combined Raman and Brillouin inelastic light scattering experiments show the local distribution of cooling rates and residual stresses (detailed behavior of the glass structure) in the interior and the surrounding of an USP laser modified zone.

Keywords

Raman spectroscopyfused silicaglass structureultra-short pulsed lasercooling ratefictive temperatureBrillouin spectroscopy

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International Journal of Extreme Manufacturing
Volume 2 Issue 3,
September 2020
Pages 035001-035001
DOI: 10.1088/2631-7990/ab9583
Cite this article:
Bergler M, Cvecek K, Werr F, et al. Cooling rate calibration and mapping of ultra-short pulsed laser modifications in fused silica by Raman and Brillouin spectroscopy. International Journal of Extreme Manufacturing, 2020, 2(3): 035001. https://doi.org/10.1088/2631-7990/ab9583

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Received: 24 February 2020
Revised: 10 April 2020
Accepted: 21 May 2020
Published: 30 June 2020
© 2020 The Author(s).

Original content from this work may be used under the terms of the Creative Commons Attribution 3.0 licence. Any further distribution of this work must maintain attribution to the author(s) and the title of the work, journal citation and DOI.
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