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Research Article | Open Access

Rapid photothermal heating of aqueous batteries for low-temperature conditions

Zhichun Yu1Jiaxing Liang1,2,3Jian Pan1Jiangtao Xu1Guojin Liang2,3Zhifang Shi2,3Wei Feng2,3Dewei Chu1( )Ruopian Fang1( )Da-Wei Wang1,2,3( )
School of Chemical Engineering, The University of New South Wales, Sydney 2052, Australia
Faculty of Materials Science and Energy Engineering, Shenzhen University of Advanced Technology, Shenzhen 518107, China
Institute of Technology for Carbon Neutrality, Shenzhen Institute of Advanced Technology, Chinese Academy of Sciences, Shenzhen 518107, China
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Abstract

Aqueous batteries are promising for large-scale applications owing to their affordability, eco-friendliness, and nonflammability. However, their usability in cold regions is limited by electrolyte freezing and slow ion-transfer kinetics at subzero temperatures. This study demonstrates the stable operation of aqueous batteries in subzero conditions by integrating high-efficiency photothermal current collectors with suspension electrodes. The Ketjen black-based photothermal current collectors efficiently convert a broad spectrum of sunlight (98%, 200–2500 nm) into thermal energy, enabling rapid heat generation. Simultaneously, the high thermal conductivity of the suspension electrode ensures quick distribution of thermal energy throughout the battery. This configuration allows the cell’s core temperature to rapidly increase from −18 °C to 20 °C within 22 min under simulated solar irradiation. Additionally, an integrated light concentrator and temperature regulation system has been developed to improve heating rates and ensure the temperature stability of the cell under various climatic conditions. As a result, the cell can maintain a stable temperature of 20 °C during consecutive charge/discharge cycles, even with an ambient temperature fluctuating between −5 °C and 5 °C. This integrated photothermal battery design exhibits great potential for cold weather conditions, paving the way for the deployment of large-scale aqueous battery systems in polar regions.

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Energy Materials and Devices
Article number: 9370043
Cite this article:
Yu Z, Liang J, Pan J, et al. Rapid photothermal heating of aqueous batteries for low-temperature conditions. Energy Materials and Devices, 2024, 2(3): 9370043. https://doi.org/10.26599/EMD.2024.9370043

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Received: 24 June 2024
Revised: 16 July 2024
Accepted: 26 July 2024
Published: 25 September 2024
© The Author(s) 2024. Published by Tsinghua University Press.

The articles published in this open access journal are distributed under the terms of the Creative Commons Attribution 4.0 International License (http://creativecommons.org/licenses/by/4.0/), which permits use, distribution and reproduction in any medium, provided the original work is properly cited.

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