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Electro-optic modulators, which convert electrical signals onto the transmission light, are key devices in electro-optic modulating systems. Modulation efficiency is one of the most important parameters of an electro-optic modulator, which directly determines the footprint and power consumption of the device. Generally, modulation efficiency strongly depends on the electro-optic response of the crystal. The Pb(In1/2Nb1/2)O3–Pb(Mg1/3Nb2/3)O3–PbTiO3 (PIN–PMN–PT) single crystal with giant electro-optic coefficient (
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