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This study introduces a novel relay and synergistic anti-corrosion mechanisms by constructing an active anticorrosive coating with nanocontainers through the combination of zinc-based zeolitic imidazolate framework materials (ZIF-8) and layered double hydroxides loaded with molybdate anions (MoO42− LDHs). The incorporation of ZIF-8 provided the material with abundant surface nano-micropores, enhancing its adsorption capacity for corrosive ions such as OH− and Cl−. Simultaneously, this adsorption enabled the ZIF-8-loaded NiAl-MoO42− LDH to receive signals induced by Cl− stimulation or pH changes. After receiving the signals, the corrosion inhibitor MoO42− encapsulated within the NiAl-MoO42− LDH was released responsively and exchanged with Cl−. The released MoO42− from nanocontainers adsorbed onto localized corrosion sites, forming a passivation film, thereby blocking the diffusion path of Cl−. Additionally, this study demonstrated that the self-assembly of ZIF-8 effectively reduced the hydrophilicity of LDH and enhanced the resistance of coating to permeability. Through supramolecular interactions between LDH hydroxyl groups, metal-organic framework (MOF) functional groups and organic epoxy resin, the cross-linking of the coating and the interfacial compatibility of the materials were significantly improved. The Z-type heterojunction composed of nickel-based LDH and metal organic frameworks not only increased the specific surface area and capacitance performance but also provided photo-induced cathodic protection for metal substrates with matched bandgaps. The experimental results showed that the impedance properties of the ZIF-8/NiAl-MoO42− LDH coatings were 28.43 times of pure epoxy after 168 h. This work can provide new insights and assistance for the study of anti-corrosion mechanisms.
Abrantes Leal, D.; Sousa, I.; Bastos, A. C.; Tedim, J.; Wypych, F.; Bruno Marino, C. E. Combination of layered-based materials as an innovative strategy for improving active corrosion protection of carbon steel. Surf. Coat. Technol. 2023, 473, 129972.
Prabhu, S.; Maruthapandi, M.; Durairaj, A.; Luong, J. H. T.; Gedanken, A. Enhanced electrochemical performance of CuO Capsules@CDs composites for solid-state hybrid supercapacitor. Energy Fuels 2023, 37, 6824–6833.
Mohammadi, I.; Izadi, M.; Shahrabi, T.; Fathi, D.; Fateh, A. Enhanced epoxy coating based on cerium loaded Na-montmorillonite as active anti-corrosive nanoreservoirs for corrosion protection of mild steel: Synthesis, characterization, and electrochemical behavior. Prog. Org. Coat. 2019, 131, 119–130.
Kim, M.; Brewer, L. N.; Kubacki, G. W. Microstructure and corrosion resistance of chromate conversion coating on cold sprayed aluminum alloy 2024. Surf. Coat. Technol. 2023, 460, 129423.
Yasakau, K. A.; Kallip, S.; Zheludkevich, M. L.; Ferreira, M. G. S. Active corrosion protection of AA2024 by sol–gel coatings with cerium molybdate nanowires. Electrochim. Acta 2013, 112, 236–246.
Abrantes Leal, D.; Wypych, F.; Bruno Marino, C. E. Zinc-layered hydroxide salt intercalated with molybdate anions as a new smart nanocontainer for active corrosion protection of carbon steel. ACS Appl. Mater. Interfaces 2020, 12, 19823–19833.
Wang, T. G.; Cao, H. J. Orientation control and characterization strategies towards developing 2D materials-based composite coatings for corrosion protection on metals: Progresses and challenges. Prog. Org. Coat. 2023, 182, 107715.
Wang, J. B.; Zhao, J. M.; Tabish, M.; Shi, F.; Fan, B. M.; Peng, L. J.; Cheng, Q. Intelligent anticorrosion coating based on mesostructured BTA@mCeO2/g-C3N4 nanocomposites for inhibiting the filiform corrosion of Zn-Mg-Al coated steel. Corros. Sci. 2023, 221, 111331.
Liu, W.; Yu, J. G.; Li, T. S.; Li, S. H.; Ding, B. Y.; Guo, X. L.; Cao, A. Q.; Sha, Q. H.; Zhou, D. J.; Kuang, Y. et al. Self-protecting CoFeAl-layered double hydroxides enable stable and efficient brine oxidation at 2 A·cm−2. Nat. Commun. 2024, 15, 4712.
Zhang, Y.; Feng, B.; Yan, M. L.; Shen, Z.; Chen, Y. Q.; Tian, J. Y.; Xu, F. F.; Chen, G. H.; Wang, X. Z.; Yang, L. J. et al. Self-supported NiFe-LDH nanosheets on NiMo-based nanorods as high-performance bifunctional electrocatalysts for overall water splitting at industrial-level current densities. Nano Res. 2024, 17, 3769–3776.
Singha Roy, S.; Karmakar, A.; Madhu, R.; Nagappan, S.; N Dhandapani, H.; Kundu, S. Three-dimensional Sm-doped NiCu-LDH on Ni foam as a highly robust bifunctional electrocatalyst for total water splitting. ACS Appl. Energy Mater. 2023, 6, 8818–8829.
Xing, X. T.; Sui, Y.; Li, Q. S.; Yuan, M.; Zhao, H. T.; Zhou, D.; Chu, X. M.; Liu, S. J.; Tang, E. J. Multifunctional ZnAl-MoO4 LDH assembled Ti3C2T x MXene composite for active/passive corrosion protection behavior of epoxy coatings. Appl. Surf. Sci. 2023, 623, 157092.
Yasakau, K. A.; Kuznetsova, A.; Maltanava, H. M.; Poznyak, S. K.; Ferreira, M. G. S.; Zheludkevich, M. L. Corrosion protection of zinc by LDH conversion coatings. Corros. Sci. 2024, 229, 111889.
Karthik Kiran, S.; Shukla, S.; Struck, A.; Saxena, S. Surface engineering of graphene oxide shells using lamellar LDH nanostructures. ACS Appl. Mater. Interfaces 2019, 11, 20232–20240.
Ahmad, E. A.; Chang, H. Y.; Al-Kindi, M.; Joshi, G. R.; Cooper, K.; Lindsay, R.; Harrison, N. M. Corrosion protection through naturally occurring films: New insights from iron carbonate. ACS Appl. Mater. Interfaces 2019, 11, 33435–33441.
Xiong, Z. Z.; Qi, Z. H.; Zhang, W. H.; Ji, M. B.; Ma, F. Q.; Ying, L. X.; Wang, G. X. Enhancing frictional and corrosion resistance performance in aluminum alloy through in situ growth of NiZnAl-LDH membrane and its modification. Surf. Interfaces 2024, 46, 104103.
Yashas, S. R.; Shivaraju, H. P.; Sandeep, S.; Kumara Swamy, N.; Gurupadayya, B. Application of yttrium molybdate tethered polypyrrole nanocomposite for the photocatalytic remediation of nitrofurantoin in water. Surf. Interfaces 2022, 32, 102102.
Chen, Y. X.; Zhou, D.; Guo, X. J.; Yang, X.; Zhao, S. R.; Lu, Y.; Liu, J. K. Improved anticorrosion performance of mixed valence Mn-modified ZnO dilute magnetic solid solution with multilevel self-assembled network structure. Nano Res. 2022, 15, 6590–6600.
Mu, X. Q.; Zhang, X. Y.; Chen, Z. Y.; Gao, Y.; Yu, M.; Chen, D.; Pan, H. Z.; Liu, S. L.; Wang, D. S.; Mu, S. C. Constructing symmetry-mismatched Ru x Fe3− x O4 heterointerface-supported Ru clusters for efficient hydrogen evolution and oxidation reactions. Nano Lett. 2024, 24, 1015–1023.
Wang, S. C.; Zhang, M. Y.; Mu, X. Q.; Liu, S. L.; Wang, D. S.; Dai, Z. H. Atomically dispersed multi-site catalysts: Bifunctional oxygen electrocatalysts boost flexible zinc-air battery performance. Energy Environ. Sci. 2024, 17, 4847–4870.
Liu, Y.; Yao, H.; Xie, Z. H.; Yu, G.; Zhong, C. J. In situ depositing a metal-organic framework film on TiO2 nanoarray toward stable photogenerated cathodic protection for nickel-coated magnesium alloy. Appl. Surf. Sci. 2023, 638, 157937.
Guo, Y.; Jiang, Z. Q.; Ying, W.; Chen, L. P.; Liu, Y. Z.; Wang, X. B.; Jiang, Z. J.; Chen, B. L.; Peng, X. S. A DNA-threaded ZIF-8 membrane with high proton conductivity and low methanol permeability. Adv. Mater. 2018, 30, 1705155.
Man, T. T.; Xu, C. X.; Liu, X. Y.; Li, D.; Tsung, C. K.; Pei, H.; Wan, Y.; Li, L. Hierarchically encapsulating enzymes with multi-shelled metal-organic frameworks for tandem biocatalytic reactions. Nat. Commun. 2022, 13, 305.
Duan, P. F.; An, Y. H.; Wei, X. X.; Tian, Y. J.; Guan, D.; Liu, X. W.; Mao, L. Q. A novel structure of ultra-high-loading small molecules-encapsulated ZIF-8 colloid particles. Nano Res. 2024, 17, 2929–2940.
Huang, Y.; Zhao, C. Y.; Li, Y.; Wang, C.; Yuan, W. L.; Shen, T.; Liu, J.; Cheng, D.; Wu, C. C.; Shen, Q. H. et al. A smart sol–gel coating incorporating pH-responsive BTA-ZIF-8 MOF assembled hexagonal boron nitride for active/passive corrosion protection of 1060 aluminum alloy. Surf. Coat. Technol. 2023, 474, 130072.
Zhong, Y.; Wu, C. L.; Jia, X. F.; Sun, S. J.; Chen, D. M.; Yao, W. Q.; Ding, H.; Zhang, J. Y.; Ma, T. Y. Coupling of self-healing atomic layer CoAl-LDH onto Mo:BiVO4 photoanode for fast surface charge transfer toward stable and high-performance water splitting. Chem. Eng. J. 2023, 465, 142893.
Fu, M. J.; Chai, B.; Zhang, X. H.; Sun, Y.; Fan, G. Z.; Song, G. S. Nitrogen self-doped chitosan carbon aerogel integrating with CoAl-LDH for ultra-efficient sulfamethoxazole degradation based on PS-AOPs: From batch to continuous process. J. Environ. Chem. Eng. 2023, 11, 110650.
Xu, J.; Li, Q.; Liu, X. Y.; Yang, Q. P-doped nanorod MoO3 and nanoflower NiAl-LDH construct S-type heterojunction for photocatalytic high-efficiency hydrogen evolution. Surf. Interfaces 2023, 43, 103593.
Li, Z. K.; Xu, Z. H.; Wang, G. S.; Ding, Y. J.; Yan, Z. X.; Yue, L. Interfacial construction promoted binder-free NiCo-LDH/Mn-ZIF on carbon cloth for high-performance supercapacitor. Electrochim. Acta 2024, 475, 143701.
Zhang, Y. Y.; Liu, H.; Zhu, P. F.; Yang, M. X.; Jin, Z. L. In situ XPS proved effective charge transfer over ZIF-67@CoFe LDH S-scheme heterojunctions for efficient visible light driven hydrogen evolution. Int. J. Hydrogen Energy 2023, 48, 32631–32641.
Wang, G. R.; Jin, Z. L.; Zhang, W. X. Ostensibly phosphatized NiAl LDHs nanoflowers with remarkable charge storage property for asymmetric supercapacitors. J. Colloid Interface Sci. 2020, 577, 115–126.
Tonda, S.; Kumar, S.; Bhardwaj, M.; Yadav, P.; Ogale, S. g-C3N4/NiAl-LDH 2D/2D hybrid heterojunction for high-performance photocatalytic reduction of CO2 into renewable fuels. ACS Appl. Mater. Interfaces 2018, 10, 2667–2678.
Sun, C.; Hu, J.; Wu, L. X.; Xia, Q. L.; Jiao, F. P. Construction of a novel visible-light-driven Z-scheme NiAl-LDH modified (BiO)2CO3 heterostructure for enhanced photocatalytic degradation antibiotics performance in natural water bodies. Ind. Eng. Chem. Res. 2023, 62, 466–477.
Liu, Q.; Zhou, F.; Bai, Y. Y.; Hu, W. K. Evaluating properties of carbon-free nano-NiCoFe-LDHs with molybdate as oxygen evolution catalysts and their applications in rechargeable air electrodes. Energy Fuels 2021, 35, 20374–20385.
Wang, H. O.; Wang, H. M.; Wang, H. F.; Su, Q. D.; Jiang, H.; Pan, Y. P.; Ma, X. F.; Hao, S. J.; Liu, J. W. β supported Fe2(MoO4)3: An efficient solid acidic heterogeneous catalyst for the synthesis of 2-ethoxyethyl acetate. Microporous Mesoporous Mater. 2024, 369, 112985.
Popov, V. V.; Menushenkov, A. P.; Yastrebtsev, A. A.; Molokova, A. Y.; Rudakov, S. G.; Svetogorov, R. D.; Tsarenko, N. A.; Ponkratov, K. V.; Ognevskaya, N. V.; Seregina, O. N. The effect of the synthesis conditions on the structure and phase transitions in Ln2(MoO4)3. Solid State Sci. 2021, 112, 106518.
Chen, X.; Fan, B. C.; Wang, H.; Liu, X. F.; Liu, Y.; Gao, J. K. Multiflower-like ReS2/NiAl-LDH heterojunction for visible-light-driven photocatalytic CO2 reduction. Inorg. Chem. 2024, 63, 5132–5141.
Kalusulingam, R.; Mariyaselvakumar, M.; Antonyraj, C. A.; Mathi, S.; Mikhailova, T. S.; Khubezhov, S. A.; Pankov, I. V.; Srinivasan, K.; Myasoedova, T. N. Highly efficient water splitting with Pd-integrated NiAl-LDH nanosheets as bifunctional electrocatalysts. Energy Fuels 2023, 37, 13319–13330.
Chaudhary, K.; Dhiman, D.; Venkatesu, P.; Masram, D. T. Classically synthesized ZIF-8 and Au/ZIF-8 for biocompatibility assessment with hemoglobin. ACS Sustain. Chem. Eng. 2022, 10, 12962–12967.
Wang, X. B.; Liu, J.; Leong, S.; Lin, X. C.; Wei, J.; Kong, B.; Xu, Y. F.; Low, Z. X.; Yao, J. F.; Wang, H. T. Rapid construction of ZnO@ZIF-8 heterostructures with size-selective photocatalysis properties. ACS Appl. Mater. Interfaces 2016, 8, 9080–9087.
Pei, X. Y.; Song, W. Y.; Zhang, Z. W.; Zhao, Y.; Li, Z. Y. CO2-responsive CuI-ionic liquid/zeolitic imidazolate frameworks stabilized Pickering emulsions for azide-alkyne click reaction. ACS Appl. Nano Mater. 2023, 6, 19972–19980.
Ding, R. J.; Zhu, H. F.; Zhou, J. S.; Luo, H. H.; Xue, K. H.; Yu, L. Q.; Zhang, Y. P. Highly water-stable and efficient hydrogen-producing heterostructure synthesized from Mn0.5Cd0.5S and a zeolitic imidazolate framework ZIF-8 via ligand and cation exchange. ACS Appl. Mater. Interfaces 2023, 15, 36477–36488.
Niu, X. H.; Yan, S. M.; Zhao, R.; Li, H. X.; Liu, X. Y.; Wang, K. J. Design and electrochemical chiral sensing of the robust sandwich chiral composite D-His-ZIF-8@Au@ZIF-8. ACS Appl. Mater. Interfaces 2023, 15, 22435–22444.
Mu, C. L.; Ren, J. H.; Chen, H.; Wu, Y.; Xu, Q. N.; Sun, X. D.; Yan, K. Graphitic carbon nitride/zeolitic imidazolate framework-8 nanoparticles with antibacterial properties for textile coating. ACS Appl. Nano Mater. 2021, 4, 10634–10644.
Jin, Z. L.; Wang, X. Y.; Wang, Y. P.; Yan, T.; Hao, X. Q. Snowflake-like Cu2S coated with NiAl-LDH forms a p–n heterojunction for efficient photocatalytic hydrogen evolution. ACS Appl. Energy Mater. 2021, 4, 14220–14231.
Ma, B. C.; Zhang, C.; Jia, D. J.; Zhao, Q. X.; Yang, P. P. NiAl-LDH-modified core–shell rod-like ZnO@ZnS heterostructures for enhanced photocatalytic hydrogen precipitation. J. Phys. Chem. C 2023, 127, 2908–2917.
Ren, R.; Liu, G. C.; Kim, J. Y.; Ardhi, R. E. A.; Tran, M. X.; Yang, W.; Lee, J. K. Photoactive g-C3N4/CuZIF-67 bifunctional electrocatalyst with staggered p–n heterojunction for rechargeable Zn-air batteries. Appl. Catal. B: Environ. 2022, 306, 121096.
Tantisriyanurak, S.; Klinyod, S.; Leangsiri, W.; Nunthakitgoson, W.; Soyphet, A.; Ketkaew, M.; Thivasasith, A.; Iadrat, P.; Rodaum, C.; Atithep, T. et al. Carbon nanotubes deposited on mordenite zeolite/NiAl-layered double hydroxide composites as electrocatalysts for 2,5-furandicarboxylic acid production from 5-hydroxymethylfurfural. ACS Appl. Nano Mater. 2023, 6, 8784–8794.
Wu, Y. L.; Zhu, P. F.; Li, Y. J.; Zhang, L. J.; Jin, Z. L. In situ derivatization of NiAl-LDH/NiS a p–n heterojunction for efficient photocatalytic hydrogen evolution. ACS Appl. Energy Mater. 2022, 5, 8157–8168.
Ma, X. L.; Zhou, L. X.; Chen, T.; Sun, P. P.; Lv, X. W.; Yu, H. Z.; Sun, X. H.; Leo Liu, T. High-performance aqueous rechargeable NiCo//Zn battery with molybdate anion intercalated CoNi-LDH@CP bilayered cathode. J. Colloid Interface Sci. 2024, 658, 728–738.
Ju, X. Q.; Yang, Z. Y.; Wang, J. W.; Cui, B. L.; Xin, Y. Y.; Zheng, Y. P.; Wang, D. C. Converting nanoflower-like layered double hydroxides into solvent-free nanofluids for CO2 capture. ACS Appl. Mater. Interfaces 2023, 15, 56181–56191.
Wang, Q. X.; Lei, Y. T.; Cui, Y. Y.; Lin, J. R. L.; Huang, W.; He, Y. Thermal stability and kinetics of single I2@ZIF-8 particles. ACS Appl. Mater. Interfaces 2022, 14, 22643–22649.
Tian, J. J.; Chen, Y. X.; Liu, Z. X.; Liu, J. K. Synthesis and mechanism of Co2+/Sr2+ codoped magnetic lanthanum cuprate with excellent corrosion resistance. ACS Appl. Mater. Interfaces 2023, 15, 53651–53664.
Liu, S. Y.; Duan, J. Q.; Zhang, M. Y.; Wang, H.; Liu, Y. X.; Chen, W. P.; Wen, H. M.; Fu, Z. Q. Correlation of microstructure, mechanical properties and corrosion behavior in a Ni34Co28Cr28Al10 multi-principal element alloy with outstanding corrosion resistance. Corros. Sci. 2024, 228, 111835.
Liu, Z. X.; Zhou, D.; Tian, J. J.; Liu, J. K. Vanadium-doped induction of bare active crystalline planes of tungsten oxide and its excellent anticorrosion properties. ACS Appl. Eng. Mater 2023, 1, 2926–2940.
Wang, Z.; Jin, Z. Y.; Liu, H. X.; Liu, R. L.; Zhang, Y.; Yin, Y. S.; Liu, H. F.; Yuan, X.; Fan, S. J.; Liu, H. W. Insights into the hydrophobic coating with integrated high-efficiency anti-corrosion, anti-biofouling and self-healing properties based on anti-bacterial nano LDH materials. Corros. Sci. 2024, 231, 111995.
Zan, G. T.; Li, S. Q.; Chen, P.; Dong, K. Z.; Wu, Q. S.; Wu, T. Mesoporous cubic nanocages assembled by coupled monolayers with 100% theoretical capacity and robust cycling. ACS Cent. Sci. 2024, 10, 1283–1294.
Song, L. Y.; Ma, X. M.; Chen, Z. Y.; Hou, B. R. The role of UV illumination on the initial atmospheric corrosion of 09CuPCrNi weathering steel in the presence of NaCl particles. Corros. Sci. 2014, 87, 427–437.
Xu, D.; Zhang, S. N.; Chen, J. S.; Li, X. H. Design of the synergistic rectifying interfaces in Mott–Schottky catalysts. Chem. Rev. 2023, 123, 1–30.
Yamasaki, T.; Iimura, S.; Kim, J.; Hosono, H. Extremely shallow valence band in lanthanum trihydride. J. Am. Chem. Soc. 2023, 145, 560–566.
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