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Research Article | Open Access

Multistage carbon coupling on three-dimensional multi-space biological templates: A novel strategy for multifunctional microwave absorption aerogel

Dashuang Wang1, Tuo Ping1,2, Zhilan Du1, Yan Liao1, Hong Gao4, Xiaobin Gong1, Jinsong Rao1, Bo Wang5, Shicheng Wei5, Xiaoying Liu3(), Yuxin Zhang1()
College of Materials Science and Engineering, Chongqing University, Chongqing 400044, China
Beijing Spacecrafts, China Academy of Space Technology, Beijing 100194, China
Army Logistics Academy of PLA, Chongqing 401331, China
China Academy of Space Technology, Beijing 100194, China
National Key Laboratory for Remanufacturing, Army Academy of Armored Forces, Bejjing 100072, China
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Utilizing magnetic–electric synergy and impedance matching effects, a novel NiCo LDH/C@Diatomite (NC/C@De) aerogel has been prepared through the coupling of porous materials and the synergistic action of multilevel carbon materials. This aerogel exhibits broadband electromagnetic wave absorption with an effective absorption bandwidth of 8.56 GHz and a reflection loss minimum of −46.85 dB at a thickness of 2.7 mm.

Abstract

Nowadays, with the dramatic development of microwave absorbing materials (MAMs), broadband and lightweight are still a topic that cannot be bypassed. Considering the drawbacks of single-component materials and the necessity of magnetic–electric synergistic effect. A novel porous carbon-based aerogel composite with a three-dimensional (3D) biological template is prepared by using rational impedance matching design and multifunctional optimization. Specifically, the coupling of porous materials as well as the synergy of multilevel carbon materials. A novel aerogel of NiCo layered double hydroxide (LDH)/C@Diatomite (De) was prepared by thermal carbonization to convert polypyrrole (PPy) into C particles deposited on the surface of magnetic LDH, coupled to form an aerogel on the basis of De carrier. The influence of the involvement of multilevel carbon on the electromagnetic wave absorption (EMWA) properties of the composites and its potential attenuation mechanism as well as the synergistic effect of the coupling of porous materials are revealed. As a result, the effective absorption bandwidth (EAB) is 8.56 GHz with a reflection loss minimum (RLmin) of −46.85 dB at a thickness of 2.7 mm. With super hydrophobicity and thermal management properties. This work not only provides inspiration for the development of new aerogel MAMs with superior performance, but also has great potential for further development and practical application.

Keywords

microwave absorptiondiatomitegraphene aerogeldelectric loss

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Nano Research
Volume 18 Issue 3,
March 2025
Article number: 94907226
DOI: 10.26599/NR.2025.94907226
Cite this article:
Wang D, Ping T, Du Z, et al. Multistage carbon coupling on three-dimensional multi-space biological templates: A novel strategy for multifunctional microwave absorption aerogel. Nano Research, 2025, 18(3): 94907226. https://doi.org/10.26599/NR.2025.94907226
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