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Research Article | Open Access

Generation of ultrathin two-dimensional MOF-derived nanocomposites based on ion-exchange strategy with enhanced microwave absorption properties

Zuolong Ning1,2, Hexia Huang1(), Yanru He3 (), Yijie Liu2, Jiaqi Tao2, Lvtong Duan2, Yucheng Wang2, Zhenyu Cheng2, Zhenglin Liu2, Jintang Zhou2
College of Energy and Power Engineering, Nanjing University of Aeronautics and Astronautics, Nanjing 210016, China
College of Materials Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing 211100, China
Southwest Technology and Engineering Research Institute, Chongqing 400039, China
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In this study, the transformation of two-dimensional (2D) templates into hollow layered double hydroxides with porous surfaces is realized by using 2D Co-based metal-organic framework (MOF) layered zeolitic imidazolate framework (ZIF-L) as a structural design template and combining it with an efficient ion-exchange component modulation method. The potential advantages of morphology design and component modulation in synergistically modulating electromagnetic parameters are fully utilized, and a significant improvement in microwave absorption properties is realized.

Abstract

Metal-organic frameworks (MOFs) materials exhibit inherent advantages in microwave absorption (MA) due to their unique compositional and structural characteristics. However, it remains a significant challenge to systematically elucidate the coordinated effects of component modulation and morphology design on electromagnetic parameters during the complex modification process to enhance the MA performance of MOFs. In this study, the two-dimensional (2D) Co-based MOFs material, layered zeolitic imidazolate framework (ZIF-L), was meticulously selected as a structure design template and combined with an efficient ion-exchange component modulation method, aiming to stimulate the potential advantages between the two in the synergistic modulation of electromagnetic parameters. Specifically, the ion-exchange method enhanced various polarization mechanisms, including interface, dipole, and defect-induced polarizations. Meanwhile, the 2D template facilitates the formation of a robust conductive network on the surface and ensures the high efficiency and uniformity of the ion-exchange process. Ultimately, the resulting material achieved an adequate absorption bandwidth (EAB) of 6.47 GHz at a thickness of 2 mm, a 78% improvement over the untreated sample (EAB = 3.64 GHz). This research not only provides valuable theoretical insights into the application of 2D MOFs materials in MA but also offers innovative perspectives for the design and development of energy-saving and environmentally friendly microwave absorption materials (MAMs).

Keywords

metal-organic frameworkblade-like layered zeolitic imidazolate framework (ZIF-L)microwave absorption

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Nano Research
Volume 18 Issue 6,
June 2025
Article number: 94907283
DOI: 10.26599/NR.2025.94907283
Cite this article:
Ning Z, Huang H, He Y, et al. Generation of ultrathin two-dimensional MOF-derived nanocomposites based on ion-exchange strategy with enhanced microwave absorption properties. Nano Research, 2025, 18(6): 94907283. https://doi.org/10.26599/NR.2025.94907283
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