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Research Article | Open Access

NiS2/FeS Heterostructured Nanoflowers for High-Performance Sodium Storage

Dong Yan1,2, Shuhao Xiao2, Xinyan Li2, Jinxia Jiang3( ), Qiyuan He4, Hanchao Li2, Jiaqian Qin5, Rui Wu2, Xiaobin Niu2, Jun Song Chen1,2,6( )
Institute for Advanced Study, Chengdu University, Chengdu 610106, P. R. China
School of Materials and Energy, University of Electronic Science and Technology of China, Chengdu 610054, P. R. China
Chongqing Medical and Pharmaceutical College, Chongqing 401331, P. R. China
Department of Materials Science and Engineering, City University of Hong Kong, Kowloon, Hong Kong, China
Center of Excellence on Advanced Materials for Energy Storage, Metallurgy and Materials Science Research Institute, Chulalongkorn University, Bangkok 10330, Thailand
Shenzhen Institute for Advanced Study, University of Electronic Science and Technology of China, Shenzhen, P. R. China
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Abstract

Transition metal sulfides demonstrate attractive potential for sodium storage owing to their high theoretical specific capacity and high reserve. However, the low conductivity and volume expansion deteriorate their high-rate performance and cycling stability. In this work, we construct NiS2/FeS heterostructure by growing Ni-based layered double hydroxide nanosheets on Fe-based Prussian Blue nanocrystals followed by gaseous sulfurization, giving rise to flower-like NiS2/FeS nanoparticles. The as-prepared nanocomposite exhibits good rate performance of 156 mAh g−1 at 50 A g−1 and long cycle life of 606 mAh g−1 at 5 A g−1 after 1,000 cycles, which are superior to the heterostructure-free counterpart of NiS2 and FeS. Density functional theory calculation further verifies that the enhanced electrochemical performance of NiS2/FeS is due to the existence of interface derived from the heterostructure.

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Energy Material Advances
Volume 4,
2023
Article number: 0012
DOI: 10.34133/energymatadv.0012
Cite this article:
Yan D, Xiao S, Li X, et al. NiS2/FeS Heterostructured Nanoflowers for High-Performance Sodium Storage. Energy Material Advances, 2023, 4: 0012. https://doi.org/10.34133/energymatadv.0012

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Received: 16 September 2022
Accepted: 14 December 2022
Published: 31 January 2023
© 2023 Dong Yan et al. Exclusive Licensee Beijing Institute of Technology Press. No claim to original U.S. Government Works.

Distributed under a Creative Commons Attribution License (CC BY 4.0).
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