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Research Article | Open Access

Coarse and fine-tuning of lasing transverse electromagnetic modes in coupled all-inorganic perovskite quantum dots

Youngsin Park1,§, Guanhua Ying2,§, Atanu Jana1,§, Vitaly Osokin2, Claudius C. Kocher2, Tristan Farrow3,2( ), Robert A. Taylor2( ), Kwang S. Kim1( )
School of Natural Science, Ulsan National Institute of Science and Technologh, Ulsan 44919, Republic of Korea
Clarendon Laboratory, Department of Physics, University of Oxford, Parks Road, Oxford, OX1 3PU, UK
Centre for Quantum Technologies, National University of Singapore, Science Drive 2, Singapore 117543, Singapore

§ Youngsin Park, Guanhua Ying, and Atanu Jana contributed equally to this work.

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Graphical Abstract

Abstract

Inorganic perovskite lasers are of particular interest, with much recent work focusing on Fabry-Pérot cavity-forming nanowires. We demonstrate the direct observation of lasing from transverse electromagnetic (TEM) modes with a long coherence time ~ 9.5 ps in coupled CsPbBr3 quantum dots, which dispense with an external cavity resonator and show how the wavelength of the modes can be controlled via two independent tuning-mechanisms. Controlling the pump power allowed us to fine-tune the TEM mode structure to the emission wavelength, thus providing a degree of control over the properties of the lasing signal. The temperature-tuning provided an additional degree of control over the wavelength of the lasing peak, importantly, maintained a constant full width at half maximum (FWHM) over the entire tuning range without mode-hopping.

Keywords

perovskite quantum dotscoherent lasingtransverse electromagnetic modestimulated emission

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Nano Research
Volume 14 Issue 1,
January 2021
Pages 108-113
DOI: 10.1007/s12274-020-3051-y
Cite this article:
Park Y, Ying G, Jana A, et al. Coarse and fine-tuning of lasing transverse electromagnetic modes in coupled all-inorganic perovskite quantum dots. Nano Research, 2021, 14(1): 108-113. https://doi.org/10.1007/s12274-020-3051-y
Topics:
Bromine compoundsCesium compoundsLead compoundsNanocrystalsPerovskiteSemiconductor quantum dots

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Received: 20 May 2020
Revised: 10 August 2020
Accepted: 11 August 2020
Published: 05 January 2021
© The Author(s) 2020

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