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Research Article

Robust double-layered ANF/MXene-PEDOT:PSS Janus films with excellent multi-source driven heating and electromagnetic interference shielding properties

Bing Zhou, Jianzhou Song, Bo Wang, Yuezhan Feng( ), Chuntai Liu( ), Changyu Shen
Key Laboratory of Materials Processing and Mold Ministry of Education, National Engineering Research Center for Advanced Polymer Processing Technology, Zhengzhou University, Zhengzhou 450002, China
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Graphical Abstract

Multifunctional aramid nanofiber (ANF)/MXene-poly(3,4-ethylenedioxy-thiophene):poly(styrenesulfonate) (PEDOT:PSS) films with double-layered Janus structure exhibited excellent comprehensive properties, including hydrophobicity, electrical conductivity, electromagnetic interference (EMI) shielding, and mechanical and multi-source driven heating properties, which should be useful for preparing advanced electronic components in future.

Abstract

The strategy of incorporating polymers into MXene-based functional materials has been widely used to improve their mechanical properties, however with inevitable sacrifice of their electrical conductivity and electromagnetic interference (EMI) shielding performance. This study demonstrates a facile yet efficient layering structure design to prepare the highly robust and conductive double-layer Janus films comprised of independent aramid nanofiber (ANF) and Ti3C2Tx MXene/poly(3,4-ethylenedioxy- thiophene):poly(styrenesulfonate) (PEDOT:PSS) layers. The ANF layer serves to provide good mechanical stability, whilst the MXene/PEDOT:PSS layer ensures excellent electrical conductivity. Doping PEDOT:PSS into the MXene layer enhances the interfacial bonding strength between the MXene and ANF layers and improves the hydrophobicity and water/oxidation resistance of MXene layer. The resultant ANF/MXene-PEDOT:PSS Janus film with a conductive layer thickness of 4.4 μm was shown to display low sheet resistance (2.18 Ω/sq), good EMI shielding effectiveness (EMI SE of 48.1 dB), high mechanical strength (155.9 MPa), and overall toughness (19.4 MJ/m3). Moreover, the excellent electrical conductivity and light absorption capacity of the MXene-PEDOT:PSS conductive layer mean that these Janus films display multi-source driven heating functions, producing excellent Joule heating (382 °C at 4 V) and photothermal conversion (59.6 °C at 100 mW/m2) properties.

Keywords

MXenedouble-layer structuremechanical propertieselectromagnetic interference (EMI) shieldingelectro-/photothermal conversion

Electronic Supplementary Material

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Nano Research
Volume 15 Issue 10,
October 2022
Pages 9520-9530
DOI: 10.1007/s12274-022-4756-x
Cite this article:
Zhou B, Song J, Wang B, et al. Robust double-layered ANF/MXene-PEDOT:PSS Janus films with excellent multi-source driven heating and electromagnetic interference shielding properties. Nano Research, 2022, 15(10): 9520-9530. https://doi.org/10.1007/s12274-022-4756-x
Topics:
Conductive films
Part of a topical collection:
EM Wave Functional Materials

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Received: 10 June 2022
Revised: 01 July 2022
Accepted: 10 July 2022
Published: 05 August 2022
© Tsinghua University Press 2022
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