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Research Article | Open Access

Boosting the piezoelectric property of relaxor ferroelectric single crystal via active manipulation of defect dipole polarization

Qingyuan Hua,1( ), Huimin Liaoa,1, Xin Liua, Li Jina, Kexin Songa, Yongyong Zhuanga, Zhuo Xua, Vladimir Ya Shurb, Xiaoyong Weia( )
Electronic Materials Research Laboratory, Key Laboratory of the Ministry of Education & International Center for Dielectric Research, School of Electronic Imformation, Xi'an Jiaotong University, Xi'an, 710049, China
School of Natural Sciences and Mathematics, Ural Federal University, Ekaterinburg, 620000, Russia

1 Contributions: Qingyuan Hu and Huimin. Liao contributed equally to this work.]]>

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Abstract

To further enhance the property of piezoelectric materials is of great significance to improve the overall performance of electro-mechanical devices. Here in this work, we propose a thermal annealing and high temperature poling approach to achieve significantly enhanced piezoelectricity in Pb(In1/2Nb1/2)O3—Pb(Mg1/3Nb2/3)O3—PbTiO3 (PIN-PMN-PT) crystals with a morphotropic phase boundary (MPB) composition. The main idea of our approach is to realize a more sufficiently polarized crystal via active manipulation of defects and orientation of defect polarization. Manipulation of defect dipoles by the high temperature poling is proved by the piezo-response force microscopy. Finally, a d33 of 3300 pC/N and a SE of 0.25% are obtained, nearly 60% higher than that of conventionally poled crystals. Moreover, such a boosting of piezoelectric property is obtained under a maintained Curie temperature. Our research not only reveals the active control of defect dipole via modified poling method in the PIN-PMN-PT crystal, but also provides a feasible strategy to further improve the property of piezoelectric materials.

Keywords

Piezoelectric propertyRelaxor ferroelectric single crystalsDefectsDefect polarization

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Journal of Materiomics
Volume 9 Issue 1,
January 2023
Pages 166-173
DOI: 10.1016/j.jmat.2022.08.004
Cite this article:
Hu Q, Liao H, Liu X, et al. Boosting the piezoelectric property of relaxor ferroelectric single crystal via active manipulation of defect dipole polarization. Journal of Materiomics, 2023, 9(1): 166-173. https://doi.org/10.1016/j.jmat.2022.08.004

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Received: 18 June 2022
Revised: 02 August 2022
Accepted: 20 August 2022
Published: 17 September 2022
© 2022 The Authors.

This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).
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