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Review | Open Access

Interface engineering of inverted wide-bandgap perovskite solar cells for tandem photovoltaics

Yang Yang†, Fengyuan Li†, Ruihao Chen( ), Hongqiang Wang( )
State Key Laboratory of Solidification Processing, Center for Nano Energy Materials, School of Materials Science and Engineering, Northwestern Polytechnical University and Shaanxi Joint Labortary of Graphene, Xi’an 710072, China

† Yang Yang and Fengyuan Li contributed equally to this work.

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Abstract

Wide-bandgap perovskite solar cells (WBG PSCs) have garnered significant research attention for their potential in tandem solar cells. However, they face challenges such as high open-circuit voltage losses and severe phase instability. These issues are primarily owing to the formation of defects, ion migration, and energy level mismatches at the interface of WBG perovskite devices. Meanwhile, inverted PSCs demonstrate superior stability potential and compatibility with tandem devices, making them the most promising application for WBG perovskite materials. Consequently, interface modulation for such devices has become imperative. In this review, from the perspective of applicability in tandem devices, we first provided a concise overview of WBG perovskite research and its efficiency progress in inverted devices. We further discussed interface carrier dynamics and the potential impact of interfaces on such device performance. Afterward, we presented a comprehensive summary of interface engineering in inverted WBG perovskite (1.60 eV–1.80 eV) solar cells. The research particularly explored both the upper and buried interfaces of WBG absorbers in the inverted PSCs, thoroughly investigating interface design strategies and outlining promising research directions. Finally, this review provides insight into the future development of interface engineering for high-performance and large-area WBG PSCs.

Keywords

wide-bandgap perovskiteinverted perovskite solar cellsburied interface engineeringsurface modification

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Energy Materials and Devices
Volume 2 Issue 1,
March 2024
Article number: 9370031
DOI: 10.26599/EMD.2024.9370031
Cite this article:
Yang Y, Li F, Chen R, et al. Interface engineering of inverted wide-bandgap perovskite solar cells for tandem photovoltaics. Energy Materials and Devices, 2024, 2(1): 9370031. https://doi.org/10.26599/EMD.2024.9370031

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Received: 20 February 2024
Revised: 06 March 2024
Accepted: 08 March 2024
Published: 28 March 2024
© The Author(s) 2024. Published by Tsinghua University Press.

The articles published in this open access journal are distributed under the terms of the Creative Commons Attribution 4.0 International License (http://creativecommons.org/licenses/by/4.0/), which permits use, distribution and reproduction in any medium, provided the original work is properly cited.
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