Sort:
Open Access Research Article Issue
Screening of low-friction two-dimensional materials from high-throughput calculations using lubricating figure of merit
Friction 2024, 12(8): 1897-1908
Published: 23 May 2024
Abstract PDF (2.7 MB) Collect
Downloads:3

Two-dimensional materials are excellent lubricants with inherent advantages. However, superlubricity has been reported for only a few of these materials. Unfortunately, other promising two-dimentional (2D) materials with different physical properties cannot be discovered or applied in production; thus, energy consumption can be greatly reduced. Here, we carry out high-throughput calculations for 1,475 2D materials and screen for low-friction materials. To set a standard, we propose, for the first time, a geometry-independent lubricating figure of merit based on the conditions for stick-slip transition and our theory of Moiré friction. For the efficient calculation of this figure of merit, an innovative approach was developed based on an improved registry index model. Through calculations, 340 materials were found to have a figure of merit lower than 10−3. Eventually, a small set of 21 materials with a figure of merit lower than 10−4 were screened out. These materials can provide diverse choices for various applications. In addition, the efficient computational approach demonstrated in this work can be used to study other stacking-dependent properties.

Review Article Issue
New materials and designs for 2D-based infrared photodetectors
Nano Research 2023, 16(2): 3074-3103
Published: 04 November 2022
Abstract PDF (10.7 MB) Collect
Downloads:121

Infrared photodetectors have attracted much attention considering their wide civil and military applications. Two-dimensional (2D) materials offer new opportunities for the development of costless, high-level integration and high-performance infrared photodetectors. With the advent of a broad investigation of infrared photodetectors based on graphene and transition metal chalcogenides (TMDs) exhibiting unique properties in recent decades, research on the better performance of 2D-based infrared photodetectors has been extended to a larger scale, including explorations of new materials and artificial structure designs. In this review, after a brief background introduction, some major working mechanisms, including the photovoltaic effect, photoconductive effect, photogating effect, photothermoelectric effect and bolometric effect, are briefly offered. Then, the discussion mainly focuses on the recent progress of three categories of 2D materials beyond graphene and TMDs. Noble transition metal dichalcogenides, black phosphorus and arsenic black phosphorous and 2D ternary compounds are great examples of explorations of mid-wavelength or even long-wavelength 2D infrared photodetectors. Then, four types of rational structure designs, including type-II band alignments, photogating-enhanced designs, surface plasmon designs and ferroelectric-enhanced designs, are discussed to further enhance the performance via diverse mechanisms, which involve the narrower-bandgap-induced interlayer exciton transition, gate modulation by trapped carriers, surface plasmon polaritons and ferroelectric polarization in sequence. Furthermore, applications including imaging, flexible devices and on-chip integration for 2D-based infrared photodetectors are introduced. Finally, a summary of the state-of-the-art research status and personal discussion on the challenges are delivered.

Total 2