External stimuli induced effective regulations of luminescent material are of significant interest in the development of smart optical devices. Here, by simply doping with Er³⁺ in the 0.94Bi_0.5Na_0.5TiO₃-0.06BaTiO₃ (BNTBT) ferroelectric host, using the bendable mica substrate, and exerting mechanical strain (bending) or light illumination (via photochromic reaction), the all-inorganic, highly-transparent and flexible Er-doped BNTBT/Mica luminescent-ferroelectric thin films were designed and fabricated, displaying strain-induced dramatically elevation of up-conversion photoluminescence (PL) intensity, suppression of PL concentration quenching, outstanding endurance and durability, convenient illumination-mediated PL quenching. And the strain-induced structural changes and local lattice distortions of the thin films were further explored through theoretical calculations and Raman measurement. Our results can supply the guidance of designing other luminescent-ferroelectric materials with controlled PL properties via easy mechanical/photo stimuli for expanding the application of multifunctional wearable memory devices.